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利用远场光纤尖端镊子捕获发光纳米颗粒。

Luminescent nanoparticle trapping with far-field optical fiber-tip tweezers.

作者信息

Decombe Jean-Baptiste, Valdivia-Valero Francisco J, Dantelle Géraldine, Leménager Godefroy, Gacoin Thierry, Colas des Francs Gérard, Huant Serge, Fick Jochen

机构信息

Univ. Grenoble Alpes, Inst NEEL, 38000 Grenoble, France.

Laboratoire Interdisciplinaire Carnot de Bourgogne (ICB), UMR 6303 CNRS-Université Bourgogne Franche-Comté, 21078 Dijon, France.

出版信息

Nanoscale. 2016 Mar 7;8(9):5334-42. doi: 10.1039/c5nr07727c.

Abstract

We report stable and reproducible trapping of luminescent dielectric YAG:Ce(3+) nanoparticles with sizes down to 60 nm using far-field dual fiber tip optical tweezers. The particles are synthesized by a specific glycothermal route followed by an original protected annealing step, resulting in significantly enhanced photostability. The tweezers properties are analyzed by studying the trapped particles residual Brownian motion using video or reflected signal records. The trapping potential is harmonic in the transverse direction to the fiber axis, but reveals interference fringes in the axial direction. Large trapping stiffness of 35 and 2 pN μm(-1) W(-1) is measured for a fiber tip-to-tip distance of 3 μm and 300 nm and 60 nm particles, respectively. The forces acting on the nanoparticles are discussed within the dipolar approximation (gradient and scattering force contributions) or exact calculations using the Maxwell Stress Tensor formalism. Prospects for trapping even smaller particles are discussed.

摘要

我们报告了使用远场双光纤尖端光镊对尺寸低至60纳米的发光介电YAG:Ce(3+)纳米颗粒进行稳定且可重复的捕获。这些颗粒通过特定的糖热法合成,随后进行原始的保护退火步骤,从而显著提高了光稳定性。通过使用视频或反射信号记录研究捕获颗粒的残余布朗运动来分析光镊特性。捕获势在与光纤轴垂直的方向上呈谐波形式,但在轴向方向上显示出干涉条纹。对于光纤尖端到尖端距离为3微米以及分别为300纳米和60纳米的颗粒,测量得到的大捕获刚度分别为35和2 pN μm(-1) W(-1)。在偶极近似(梯度和散射力贡献)范围内或使用麦克斯韦应力张量形式进行精确计算,讨论了作用在纳米颗粒上的力。还讨论了捕获甚至更小颗粒的前景。

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