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在双态闪烁势驱动下磁性胶体的增强扩散和反常输运

Enhanced diffusion and anomalous transport of magnetic colloids driven above a two-state flashing potential.

作者信息

Tierno Pietro, Shaebani M Reza

机构信息

Departament d'Estructura i Constituents de la Matèria, Universitat de Barcelona, 08028 Barcelona, Spain.

出版信息

Soft Matter. 2016 Apr 14;12(14):3398-405. doi: 10.1039/c6sm00237d. Epub 2016 Mar 3.

Abstract

We combine experiments and theory to investigate the diffusive and the subdiffusive dynamics of paramagnetic colloids driven above a two-state flashing potential. The magnetic potential was realized by periodically modulating the stray field of a magnetic bubble lattice in a uniaxial ferrite garnet film. At large amplitudes H0 of the driving field, the dynamics of the particle resemble an ordinary random walk with a frequency-dependent diffusion coefficient. However, subdiffusive and oscillatory dynamics at short time scales are observed when decreasing H0. We present a persistent random walk model to elucidate the underlying mechanism of motion, and perform numerical simulations to demonstrate that the anomalous motion originates from the dynamic disorder in the structure of the magnetic lattice, induced by the slightly irregular shape of bubbles.

摘要

我们结合实验和理论来研究在双态闪烁势驱动下顺磁胶体的扩散和亚扩散动力学。通过周期性调制单轴铁氧体石榴石薄膜中磁泡点阵的杂散场来实现磁势。在驱动场的大振幅(H_0)下,粒子的动力学类似于具有频率依赖扩散系数的普通随机游走。然而,当降低(H_0)时,在短时间尺度上观察到亚扩散和振荡动力学。我们提出一个持续随机游走模型来阐明运动的潜在机制,并进行数值模拟以证明异常运动源于由气泡形状略有不规则引起的磁晶格结构中的动态无序。

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