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再悬浮技术对沉积物和悬浮颗粒物中重金属分布的影响。

Effect of the resuspension technique on distribution of the heavy metals in sediment and suspended particulate matter.

作者信息

Pourabadehei Mehdi, Mulligan Catherine N

机构信息

Department of Building, Civil and Environmental Engineering, Concordia University, 1455 de Maisonneuve Blvd. W., Montreal H3G 1M8, QC, Canada.

Department of Building, Civil and Environmental Engineering, Concordia University, 1455 de Maisonneuve Blvd. W., Montreal H3G 1M8, QC, Canada.

出版信息

Chemosphere. 2016 Jun;153:58-67. doi: 10.1016/j.chemosphere.2016.03.026. Epub 2016 Mar 21.

Abstract

Harbour areas play important roles in the economy worldwide. Human activities, however, in those areas, generate contamination, which mostly accumulates in sediments. On the other hand, harbour areas have been facing deposition of significant amounts of sediment each year. As a consequence, shallowness and accumulation of contaminants in sediment become challenging issues in harbours. Among the various management options for remediation of contaminated sediments in harbours, resuspension technique was introduced as a new approach to address those issues. The concept of the resuspension method is that finer sediments have a greater tendency to adsorb the contamination. Therefore, removing the finer sediments instead of dredging the whole contaminated area is the main goal of the resuspension technique. The objective of this paper was to evaluate the effect of the resuspension method on reducing the concentration of contamination and distribution of heavy metals in sediment and suspended particulate matter. The resuspension method was successful in reducing the concentration of seven selected heavy metals (Cr, Ni, Cu, Zn, As, Cd and Pb) by removing just 4% of the contaminated sediment. The contamination intensity in the sediment, presented by geoaccumulation index, was reduced for Cd and Pb as the main contaminants by 26 and 28 percent and the rest of the selected heavy metals returned to the natural level. The results of the sequential extraction tests and enrichment factor implied that the resuspension technique is capable of decreasing the risk of remobilization of heavy metals in the aquatic ecosystem.

摘要

港区在全球经济中发挥着重要作用。然而,这些区域的人类活动会产生污染,其中大部分会累积在沉积物中。另一方面,港区每年都面临着大量沉积物的淤积。因此,沉积物的浅化和污染物的积累成为港区面临的具有挑战性的问题。在港区受污染沉积物修复的各种管理选项中,重新悬浮技术作为解决这些问题的一种新方法被引入。重新悬浮方法的概念是,较细的沉积物更倾向于吸附污染物。因此,去除较细的沉积物而不是疏浚整个受污染区域是重新悬浮技术的主要目标。本文的目的是评估重新悬浮方法对降低沉积物和悬浮颗粒物中污染物浓度以及重金属分布的影响。通过仅去除4%的受污染沉积物,重新悬浮方法成功降低了七种选定重金属(铬、镍、铜、锌、砷、镉和铅)的浓度。以地积累指数表示的沉积物中的污染强度,作为主要污染物的镉和铅分别降低了26%和28%,其余选定的重金属恢复到自然水平。连续提取试验和富集因子的结果表明,重新悬浮技术能够降低水生生态系统中重金属再活化的风险。

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