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硬盘中受限于狭窄通道的流体的类玻璃行为。

Glasslike behavior of a hard-disk fluid confined to a narrow channel.

机构信息

School of Physics and Astronomy, University of Manchester, Manchester M13 9PL, United Kingdom.

出版信息

Phys Rev E. 2016 Mar;93(3):032101. doi: 10.1103/PhysRevE.93.032101. Epub 2016 Mar 1.

Abstract

Disks moving in a narrow channel have many features in common with the glassy behavior of hard spheres in three dimensions. In this paper we study the caging behavior of the disks that sets in at characteristic packing fraction ϕ(d). Four-point overlap functions similar to those studied when investigating dynamical heterogeneities have been determined from event-driven molecular dynamics simulations and the time-dependent dynamical length scale has been extracted from them. The dynamical length scale increases with time and, on the equilibration time scale, it is proportional to the static length scale associated with the zigzag ordering in the system, which grows rapidly above ϕ(d). The structural features responsible for the onset of caging and the glassy behavior are easy to identify as they show up in the structure factor, which we have determined exactly from the transfer-matrix approach.

摘要

在狭窄通道中运动的磁盘与三维硬球的玻璃态行为有许多共同特征。在本文中,我们研究了磁盘的笼蔽行为,这种行为在特征填充分数 ϕ(d)处出现。从事件驱动的分子动力学模拟中确定了类似于研究动力学非均匀性时研究的四点重叠函数,并从它们中提取了时变动力学长度尺度。动力学长度尺度随时间增加,在平衡时间尺度上,它与系统中之字形有序相关的静态长度尺度成正比,在 ϕ(d)以上迅速增长。导致笼蔽和玻璃化行为开始的结构特征很容易识别,因为它们出现在结构因子中,我们已经通过传递矩阵方法精确地确定了结构因子。

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