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覆盖薄液层的自推进表面活性剂颗粒群体中的模式不稳定性和动态模式。

Mode instabilities and dynamic patterns in a colony of self-propelled surfactant particles covering a thin liquid layer.

作者信息

Pototsky Andrey, Thiele Uwe, Stark Holger

机构信息

Department of Mathematics, Faculty of Science Engineering and Technology, Swinburne University of Technology, 3122, Hawthorn, Victoria, Australia.

Institut für Theoretische Physik, Westfälische Wilhelms-Universität Münster, Wilhelm Klemm Str. 9, 48149, Münster, Germany.

出版信息

Eur Phys J E Soft Matter. 2016 May;39(5):51. doi: 10.1140/epje/i2016-16051-4. Epub 2016 May 6.

Abstract

We consider a colony of point-like self-propelled surfactant particles (swimmers) without direct interactions that cover a thin liquid layer on a solid support. The particles predominantly swim normal to the free film surface with only a small component parallel to the film surface. The coupled dynamics of the swimmer density and film height profile is captured in a long-wave model allowing for diffusive and convective transport of the swimmers (including rotational diffusion). The dynamics of the film height profile is determined by i) the upward pushing force of the swimmers onto the liquid-gas interface, ii) the solutal Marangoni force due to gradients in the swimmer concentration, and iii) the rotational diffusion of the swimmers together with the in-plane active motion. After reviewing and extending the analysis of the linear stability of the uniform state, we analyse the fully nonlinear dynamic equations and show that point-like swimmers, which only interact via long-wave deformations of the liquid film, self-organise in highly regular (standing, travelling, and modulated waves) and various irregular patterns.

摘要

我们考虑一群点状的自驱动表面活性剂颗粒(游动体),它们没有直接相互作用,覆盖在固体支撑物上的一层薄液层。这些颗粒主要垂直于自由膜表面游动,只有一小部分平行于膜表面。游动体密度和膜高度分布的耦合动力学在一个长波模型中得以体现,该模型考虑了游动体的扩散和对流输运(包括旋转扩散)。膜高度分布的动力学由以下因素决定:i)游动体对液 - 气界面的向上推力;ii)由于游动体浓度梯度产生的溶质马兰戈尼力;iii)游动体的旋转扩散以及面内的主动运动。在回顾并扩展了对均匀态线性稳定性的分析之后,我们分析了完全非线性动力学方程,并表明仅通过液膜长波变形相互作用的点状游动体能够自组织成高度规则的(驻波、行波和调制波)以及各种不规则模式。

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