Do Thi-Nga, Shih Po-Hsin, Chang Cheng-Peng, Lin Chiun-Yan, Lin Ming-Fa
Department of Physics, National Cheng Kung University, Tainan, Taiwan.
Center for General Education, Tainan University of Technology, Tainan, Taiwan.
Phys Chem Chem Phys. 2016 Jun 29;18(26):17597-605. doi: 10.1039/c6cp02275h.
A generalized tight-binding model is developed to investigate the feature-rich magneto-optical properties of AAB-stacked trilayer graphene. Three intragroup and six intergroup inter-Landau-level (inter-LL) optical excitations largely enrich magneto-absorption peaks. In general, the former are much higher than the latter, depending on the phases and amplitudes of LL wavefunctions. The absorption spectra exhibit single- or twin-peak structures which are determined by quantum modes, LL energy spectra and Fermion distribution. The splitting LLs, with different localization centers (2/6 and 4/6 positions in a unit cell), can generate very distinct absorption spectra. There exist extra single peaks because of LL anti-crossings. AAB, AAA, ABA, and ABC stackings considerably differ from one another in terms of the inter-LL category, frequency, intensity, and structure of absorption peaks. The main characteristics of LL wavefunctions and energy spectra and the Fermi-Dirac function are responsible for the configuration-enriched magneto-optical spectra.
开发了一种广义紧束缚模型,以研究AAB堆叠三层石墨烯丰富的磁光特性。三个组内和六个组间的朗道能级间(inter-LL)光学激发极大地丰富了磁吸收峰。一般来说,前者比后者高得多,这取决于朗道能级波函数的相位和振幅。吸收光谱呈现出由量子模式、朗道能级能谱和费米子分布决定的单峰或双峰结构。具有不同局域中心(晶胞中的2/6和4/6位置)的分裂朗道能级可以产生非常不同的吸收光谱。由于朗道能级的反交叉,存在额外的单峰。AAB、AAA、ABA和ABC堆叠在朗道能级间类别、频率、强度和吸收峰结构方面彼此有很大差异。朗道能级波函数和能谱的主要特征以及费米-狄拉克函数是导致构型丰富的磁光谱的原因。