光催化剂上NH对NO的选择性催化还原（光催化选择性催化还原）：机理研究与进展
Selective Catalytic Reduction of NO by NH over Photocatalysts (Photo-SCR): Mechanistic Investigations and Developments.
作者信息
Yamamoto Akira, Teramura Kentaro, Tanaka Tsunehiro
机构信息
Department of Molecular Engineering Graduate School of Engineering, Kyoto University Kyoto Daigaku Katsura, Nishikyo-ku, Kyoto 615-8510, Japan.
Elements Strategy Initiative for Catalysts and Batteries (ESICB), Kyoto University Kyoto Daigaku Katsura, Nishikyo-ku, Kyoto 615-8520, Japan.
出版信息
Chem Rec. 2016 Oct;16(5):2268-2277. doi: 10.1002/tcr.201600041. Epub 2016 Jun 24.
This account describes the work of our group in the selective catalytic reduction of nitrogen oxides (NO ) with ammonia over heterogeneous photocatalysts (photo-SCR) in the past 16 years. We have found that the photo-SCR proceeds over heterogeneous photocatalysts using a gas flow reactor, elucidated the reaction mechanism under UV- and visible-light irradiation by spectroscopic and kinetic studies, and developed a highly active photo-SCR system by improving the photocatalyst material itself and the reaction system with several approaches based on the reaction mechanism.
本报告描述了我们小组在过去16年中在非均相光催化剂上用氨选择性催化还原氮氧化物（NO）（光催化选择性催化还原）方面的工作。我们发现，光催化选择性催化还原在使用气流反应器的非均相光催化剂上进行，通过光谱和动力学研究阐明了紫外光和可见光照射下的反应机理，并基于反应机理通过几种方法改进光催化剂材料本身和反应体系，开发了一种高活性的光催化选择性催化还原系统。
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