Bansal Sunil, Durrett Timothy P
Department of Biochemistry and Molecular Biophysics, Kansas State University, 141 Chalmers Hall, Manhattan, KS, 66506, USA.
Lipids. 2016 Sep;51(9):1093-102. doi: 10.1007/s11745-016-4179-0. Epub 2016 Aug 6.
Acetyl-triacylglycerols (acetyl-TAG) possess an sn-3 acetate group, which confers useful chemical and physical properties to these unusual triacylglycerols (TAG). Current methods for quantification of acetyl-TAG are time consuming and do not provide any information on the molecular species profile. Electrospray ionization mass spectrometry (ESI-MS)-based methods can overcome these drawbacks. However, the ESI-MS signal intensity for TAG depends on the aliphatic chain length and unsaturation index of the molecule. Therefore response factors for different molecular species need to be determined before any quantification. The effects of the chain length and the number of double-bonds of the sn-1/2 acyl groups on the signal intensity for the neutral loss of short chain length sn-3 groups were quantified using a series of synthesized sn-3 specific structured TAG. The signal intensity for the neutral loss of the sn-3 acyl group was found to negatively correlated with the aliphatic chain length and unsaturation index of the sn-1/2 acyl groups. The signal intensity of the neutral loss of the sn-3 acyl group was also negatively correlated with the size of that chain. Further, the position of the group undergoing neutral loss was also important, with the signal from an sn-2 acyl group much lower than that from one located at sn-3. Response factors obtained from these analyses were used to develop a method for the absolute quantification of acetyl-TAG. The increased sensitivity of this ESI-MS-based approach allowed successful quantification of acetyl-TAG in various biological settings, including the products of in vitro enzyme activity assays.
乙酰基三酰甘油(acetyl-TAG)具有一个sn-3位的乙酰基,这赋予了这些特殊的三酰甘油(TAG)有用的化学和物理性质。目前用于定量乙酰基三酰甘油的方法耗时且无法提供任何关于分子种类分布的信息。基于电喷雾电离质谱(ESI-MS)的方法可以克服这些缺点。然而,TAG的ESI-MS信号强度取决于分子的脂肪链长度和不饱和度指数。因此,在进行任何定量之前,需要确定不同分子种类的响应因子。使用一系列合成的sn-3位特异性结构TAG,对sn-1/2位酰基的链长和双键数量对短链长度sn-3位基团中性丢失信号强度的影响进行了定量。发现sn-3位酰基中性丢失的信号强度与sn-1/2位酰基的脂肪链长度和不饱和度指数呈负相关。sn-3位酰基中性丢失的信号强度也与该链的大小呈负相关。此外,发生中性丢失的基团的位置也很重要,sn-2位酰基的信号远低于位于sn-3位的酰基。从这些分析中获得的响应因子被用于开发一种乙酰基三酰甘油绝对定量的方法。这种基于ESI-MS方法的灵敏度提高,使得能够成功地定量各种生物环境中的乙酰基三酰甘油,包括体外酶活性测定的产物。