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过滤速度对生物曝气滤池处理微污染地表水过程中溶解性有机氮变化的影响

Influence of filtration velocity on DON variation in BAF for micropolluted surface water treatment.

作者信息

Ma Teng-Fei, Chen You-Peng, Kang Jia, Gao Xu, Guo Jin-Song, Fang Fang, Zhang Xiao-Tian

机构信息

Key Laboratory of the Three Gorges Reservoir Region's Eco-Environments of MOE, Chongqing University, Chongqing, 400045, China.

Key Laboratory of Reservoir Aquatic Environment of CAS, Chongqing Institute of Green and Intelligent Technology, Chinese Academy of Sciences, Chongqing, 400714, China.

出版信息

Environ Sci Pollut Res Int. 2016 Dec;23(23):23415-23421. doi: 10.1007/s11356-016-7578-0. Epub 2016 Sep 9.

Abstract

Biological aerated filters (BAFs) are widely used for the treatment of micropolluted surface water. However, the biological process produces dissolved organic nitrogen (DON), which, as precursors of nitrogenous disinfection by-products, pose potential threats to drinking water safety. Therefore, to control DON in BAF effluent, it is necessary to study the influence of BAF operation parameters on DON production. In this study, the influence of filtration velocity in a BAF on DON production was investigated. Under different filtration velocity (0.5, 2, and 4 m/h) conditions, profiles of DON concentrations along the media layer were measured. The profile at a filtration velocity of 0.5 m/h showed a decreasing trend, and the ones under filtration velocities of 2 and 4 m/h fluctuated in a small range (from 0.1 to 0.4 mg/L). Moreover, the relatively high filtration velocities of 2 and 4 m/h resulted in a lower level of DON concentration. Additionally, 3D excitation-emission matrix fluorescence spectroscopy was used to characterize DON. It is found that the patterns of DON at a relatively high filtration velocity condition (4 m/h) were obviously different from the ones under low filtration velocity conditions (0.5 and 2 m/h).

摘要

曝气生物滤池(BAF)被广泛用于处理微污染地表水。然而,生物过程会产生溶解性有机氮(DON),作为含氮消毒副产物的前体,对饮用水安全构成潜在威胁。因此,为了控制曝气生物滤池出水中的溶解性有机氮,有必要研究曝气生物滤池运行参数对溶解性有机氮产生的影响。在本研究中,研究了曝气生物滤池中过滤速度对溶解性有机氮产生的影响。在不同过滤速度(0.5、2和4米/小时)条件下,测量了溶解性有机氮浓度沿介质层的分布。过滤速度为0.5米/小时时的分布呈下降趋势,过滤速度为2和4米/小时时的分布在小范围内波动(从0.1到0.4毫克/升)。此外,2和4米/小时的较高过滤速度导致溶解性有机氮浓度较低。此外,采用三维激发-发射矩阵荧光光谱法对溶解性有机氮进行表征。研究发现,较高过滤速度条件(4米/小时)下的溶解性有机氮模式与较低过滤速度条件(0.5和2米/小时)下的明显不同。

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