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二维NbSe₂中电子相变的门控调谐

Gate Tuning of Electronic Phase Transitions in Two-Dimensional NbSe_{2}.

作者信息

Xi Xiaoxiang, Berger Helmuth, Forró László, Shan Jie, Mak Kin Fai

机构信息

Department of Physics and Center for 2-Dimensional and Layered Materials, The Pennsylvania State University, University Park, Pennsylvania 16802-6300, USA.

Institute of Condensed Matter Physics, Ecole Polytechnique Fédérale de Lausanne, 1015 Lausanne, Switzerland.

出版信息

Phys Rev Lett. 2016 Sep 2;117(10):106801. doi: 10.1103/PhysRevLett.117.106801. Epub 2016 Aug 29.

Abstract

Recent experimental advances in atomically thin transition metal dichalcogenide (TMD) metals have unveiled a range of interesting phenomena including the coexistence of charge-density-wave (CDW) order and superconductivity down to the monolayer limit. The atomic thickness of two-dimensional (2D) TMD metals also opens up the possibility for control of these electronic phase transitions by electrostatic gating. Here, we demonstrate reversible tuning of superconductivity and CDW order in model 2D TMD metal NbSe_{2} by an ionic liquid gate. A variation up to ∼50% in the superconducting transition temperature has been observed. Both superconductivity and CDW order can be strengthened (weakened) by increasing (reducing) the carrier density in 2D NbSe_{2}. The doping dependence of these phase transitions can be understood as driven by a varying electron-phonon coupling strength induced by the gate-modulated carrier density and the electronic density of states near the Fermi surface.

摘要

近期在原子级薄的过渡金属二硫属化物(TMD)金属方面的实验进展揭示了一系列有趣的现象,包括电荷密度波(CDW)序和超导性在单层极限下的共存。二维(2D)TMD金属的原子厚度也为通过静电门控控制这些电子相变开辟了可能性。在此,我们展示了通过离子液体门控对模型二维TMD金属NbSe₂中的超导性和CDW序进行可逆调节。已观察到超导转变温度变化高达约50%。通过增加(降低)二维NbSe₂中的载流子密度,可以增强(减弱)超导性和CDW序。这些相变的掺杂依赖性可以理解为由门控调制的载流子密度和费米表面附近的电子态密度所诱导的变化的电子 - 声子耦合强度驱动。

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