Brenneis Andreas, Schade Felix, Drieschner Simon, Heimbach Florian, Karl Helmut, Garrido Jose A, Holleitner Alexander W
Walter Schottky Institut and Physics Department, Technical University Munich, Am Coulombwall 4a, 85748 Garching, Germany.
Nanosystems Initiative Munich (NIM), Schellingstr. 4, 80799 Munich, Germany.
Sci Rep. 2016 Oct 20;6:35654. doi: 10.1038/srep35654.
For future on-chip communication schemes, it is essential to integrate nanoscale materials with an ultrafast optoelectronic functionality into high-frequency circuits. The atomically thin graphene has been widely demonstrated to be suitable for photovoltaic and optoelectronic devices because of its broadband optical absorption and its high electron mobility. Moreover, the ultrafast relaxation of photogenerated charge carriers has been verified in graphene. Here, we show that dual-gated graphene junctions can be functional parts of THz-circuits. As the underlying optoelectronic process, we exploit ultrafast photo-thermoelectric currents. We describe an immediate photo-thermoelectric current of the unbiased device following a femtosecond laser excitation. For a picosecond time-scale after the optical excitation, an additional photo-thermoelectric contribution shows up, which exhibits the fingerprint of a spatially inverted temperature profile. The latter can be understood by the different time-constants and thermal coupling mechanisms of the electron and phonon baths within graphene to the substrate and the metal contacts. The interplay of the processes gives rise to ultrafast electromagnetic transients in high-frequency circuits, and it is equally important for a fundamental understanding of graphene-based ultrafast photodetectors and switches.
对于未来的片上通信方案,将具有超快光电功能的纳米级材料集成到高频电路中至关重要。原子级薄的石墨烯因其宽带光吸收和高电子迁移率,已被广泛证明适用于光伏和光电器件。此外,石墨烯中光生载流子的超快弛豫也已得到证实。在此,我们表明双栅极石墨烯结可以成为太赫兹电路的功能部件。作为潜在的光电过程,我们利用超快光热电流。我们描述了飞秒激光激发后无偏置器件的即时光热电流。在光激发后的皮秒时间尺度上,会出现额外的光热贡献,其呈现出空间反转温度分布的特征。后者可以通过石墨烯内电子和声子浴与衬底及金属接触的不同时间常数和热耦合机制来理解。这些过程的相互作用在高频电路中产生超快电磁瞬变,对于基于石墨烯的超快光电探测器和开关的基本理解同样重要。