Lin Jie, Jorjadze Ivane, Pontani Lea-Laetitia, Wyart Matthieu, Brujic Jasna
Center for Soft Matter Research, Department of Physics, New York University, New York, New York 10003, USA.
School of Engineering and Applied Sciences, Harvard University, Cambridge, Massachusetts 02138, USA.
Phys Rev Lett. 2016 Nov 11;117(20):208001. doi: 10.1103/PhysRevLett.117.208001. Epub 2016 Nov 8.
We report the first measurements of the effect of pressure on vibrational modes in emulsions, which serve as a model for soft frictionless spheres at zero temperature. As a function of the applied pressure, we find that the density of states D(ω) exhibits a low-frequency cutoff ω^{}, which scales linearly with the number of extra contacts per particle δz. Moreover, for ω<ω^{}, our results are consistent with D(ω)∼ω^{2}/ω^{*2}, a quadratic behavior whose prefactor is larger than what is expected from Debye theory. This surprising result agrees with recent theoretical findings [E. DeGiuli, A. Laversanne-Finot, G. A. Düring, E. Lerner, and M. Wyart, Soft Matter 10, 5628 (2014); S. Franz, G. Parisi, P. Urbani, and F. Zamponi, Proc. Natl. Acad. Sci. U.S.A. 112, 14539 (2015)]. Finally, the degree of localization of the softest low frequency modes increases with compression, as shown by the participation ratio as well as their spatial configurations. Overall, our observations show that emulsions are marginally stable and display non-plane-wave modes up to vanishing frequencies.
我们报告了压力对乳液中振动模式影响的首次测量结果,乳液可作为零温度下软无摩擦球体的模型。作为外加压力的函数,我们发现态密度D(ω)呈现出一个低频截止ω*,它与每个粒子的额外接触数δz呈线性比例关系。此外,对于ω<ω*,我们的结果与D(ω)∼ω²/ω*²一致,这是一种二次行为,其系数大于德拜理论的预期值。这一惊人结果与最近的理论发现相符[E. 德朱利、A. 拉韦尔桑 - 菲诺、G. A. 迪林、E. 勒纳和M. 怀亚特,《软物质》10, 5628 (2014); S. 弗兰兹、G. 帕里西、P. 乌尔巴尼和F. 赞波尼,《美国国家科学院院刊》112, 14539 (2015)]。最后,最软低频模式的局域化程度随着压缩而增加,这通过参与率及其空间构型得以体现。总体而言,我们的观察结果表明乳液处于临界稳定状态,并且在频率趋近于零时仍显示非平面波模式。