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通过超低本底正比计数法同时测量氚和放射性碳。

Simultaneous measurement of tritium and radiocarbon by ultra-low-background proportional counting.

作者信息

Mace Emily, Aalseth Craig, Alexander Tom, Back Henning, Day Anthony, Hoppe Eric, Keillor Martin, Moran Jim, Overman Cory, Panisko Mark, Seifert Allen

机构信息

Pacific Northwest National Laboratory, 902 Battelle Blvd, MSIN J4-65, Richland, WA 99352, USA.

Pacific Northwest National Laboratory, 902 Battelle Blvd, MSIN J4-65, Richland, WA 99352, USA.

出版信息

Appl Radiat Isot. 2017 Aug;126:171-174. doi: 10.1016/j.apradiso.2016.12.033. Epub 2016 Dec 21.

Abstract

Use of ultra-low-background capabilities at Pacific Northwest National Laboratory provide enhanced sensitivity for measurement of low-activity sources of tritium and radiocarbon using proportional counters. Tritium levels are nearly back to pre-nuclear test backgrounds (~2-8 TU in rainwater), which can complicate their dual measurement with radiocarbon due to overlap in the beta decay spectra. We present results of single-isotope proportional counter measurements used to analyze a dual-isotope methane sample synthesized from ~120mg of HO and present sensitivity results.

摘要

太平洋西北国家实验室利用超低本底能力,使用正比计数器对低活度氚源和放射性碳进行测量时,能提高测量灵敏度。氚水平几乎已恢复到核试验前的本底水平(雨水中约2 - 8 TU),由于β衰变谱重叠,这会使它们与放射性碳的双重测量变得复杂。我们展示了用于分析由约120毫克水合成的双同位素甲烷样品的单同位素正比计数器测量结果,并给出了灵敏度结果。

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