CAS Key Laboratory of Soft Matter Chemistry, and Department of Polymer Science and Engineering, University of Science and Technology of China, Hefei, Anhui Province 230026, P. R. China.
Soft Matter. 2017 Jan 25;13(4):758-764. doi: 10.1039/c6sm02679f.
A numerical investigation of the target search dynamics of self-propelled particles (SPPs) in heterogeneous environments is presented in this work. We show that the spatial heterogeneity has a dramatic effect on the target search dynamics of SPPs. The relative magnitude of the self-propulsion length l and the radius of the circular domain R determines how the mean search time of SPPs τ depends on the area fraction of fixed obstacles ϕ. For l < R, the target search process is diffusion-dominated so that a monotonic increase in τ with increasing ϕ is observed. For l > R, τ is shown to be a non-monotonic convex function as a function of ϕ due to the interplay of the distribution-dominated and diffusion-dominated dynamic regimes. Furthermore, at fixed ϕ, τ shows a minimum upon increasing the self-propulsion velocity v of a SPP of a slow rotational diffusion when it searches for a target at low ϕ, while it decreases monotonically at high ϕ. The present work highlights that the introduction of spatial heterogeneity causes rich dynamic behaviors of a SPP searching for a target, and deepens our understanding of the transport of active matter in heterogeneous media.
本文对在非均匀环境中自主运动粒子 (SPP) 的目标搜索动力学进行了数值研究。结果表明,空间非均匀性对 SPP 的目标搜索动力学有显著影响。自主运动长度 l 和圆形区域半径 R 的相对大小决定了 SPP 的平均搜索时间 τ 如何随固定障碍物的面积分数 ϕ 而变化。当 l < R 时,目标搜索过程由扩散主导,因此 τ 随着 ϕ 的增加而单调增加。当 l > R 时,由于分布主导和扩散主导的动态状态的相互作用,τ 表现为非单调凸函数。此外,在固定 ϕ 的情况下,当 SPP 以缓慢的旋转扩散速度 v 搜索目标时,τ 在低 ϕ 时出现最小值,而在高 ϕ 时单调下降。本工作强调了引入空间非均匀性会导致 SPP 搜索目标时出现丰富的动态行为,加深了我们对活性物质在非均匀介质中输运的理解。