Audier Xavier, Balla Naveen, Rigneault Hervé
Opt Lett. 2017 Jan 15;42(2):294-297. doi: 10.1364/OL.42.000294.
We demonstrate femtosecond pump-probe transient absorption spectroscopy using a programmable dispersive filter as an ultra-fast delay line. Combined with fast synchronous detection, this delay line allows for recording of 6 ps decay traces at 34 kHz. With such acquisition speed, we perform single point pump-probe spectroscopy on bulk samples in 80 μs and hyperspectral pump-probe imaging over a field of view of 100 μm in less than a second. The usability of the method is illustrated in a showcase experiment to image and discriminate between two pigments in a mixture.
我们展示了使用可编程色散滤波器作为超快延迟线的飞秒泵浦-探测瞬态吸收光谱技术。结合快速同步检测,该延迟线能够以34 kHz的频率记录6 ps的衰减轨迹。凭借这样的采集速度,我们在80 μs内对块状样品进行单点泵浦-探测光谱分析,并在不到一秒的时间内对100 μm视场进行超光谱泵浦-探测成像。在一个展示实验中,我们通过成像和区分混合物中的两种色素来说明该方法的实用性。