Dupont Maxime, Capponi Sylvain, Laflorencie Nicolas
Laboratoire de Physique Théorique, IRSAMC, Université de Toulouse, CNRS, 31062 Toulouse, France.
Phys Rev Lett. 2017 Feb 10;118(6):067204. doi: 10.1103/PhysRevLett.118.067204. Epub 2017 Feb 9.
Building on recent NMR experiments [A. Orlova et al., Phys. Rev. Lett. 118, 067203 (2017).PRLTAO0031-900710.1103/PhysRevLett.118.067203], we theoretically investigate the high magnetic field regime of the disordered quasi-one-dimensional S=1 antiferromagnetic material Ni(Cl_{1-x}Br_{x}){2}-4SC(NH{2})_{2}. The interplay between disorder, chemically controlled by Br-doping, interactions, and the external magnetic field, leads to a very rich phase diagram. Beyond the well-known antiferromagnetically ordered regime, an analog of a Bose condensate of magnons, which disappears when H≥12.3 T, we unveil a resurgence of phase coherence at a higher field H∼13.6 T, induced by the doping. Interchain couplings stabilize the finite temperature long-range order whose extension in the field-temperature space is governed by the concentration of impurities x. Such a "minicondensation" contrasts with previously reported Bose-glass physics in the same regime and should be accessible to experiments.
基于最近的核磁共振实验[A. 奥尔洛娃等人,《物理评论快报》118, 067203 (2017年)。PRLTAO0031 - 900710.1103/PhysRevLett.118.067203],我们从理论上研究了无序准一维S = 1反铁磁材料Ni(Cl₁₋ₓBrₓ)₂ - 4SC(NH₂)₂在高磁场区域的情况。由溴掺杂化学控制的无序、相互作用和外部磁场之间的相互作用,导致了一个非常丰富的相图。除了众所周知的反铁磁有序区域,即一种磁振子玻色凝聚体(当H≥12.3 T时消失)之外,我们还揭示了在更高磁场H∼13.6 T时,由掺杂诱导的相位相干的复苏。链间耦合稳定了有限温度下的长程序,其在磁场 - 温度空间中的扩展由杂质浓度x决定。这种“微凝聚”与之前报道的同一区域的玻色玻璃物理情况形成对比,并且应该可以通过实验实现。