Gu Zhi-Gang, Zhang De-Xiang, Fu Wen-Qiang, Fu Zhi-Hua, Vohra M Ismail, Zhang Lei, Wöll Christof, Zhang Jian
State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences , 350002 Fuzhou, P. R. China.
Institute of Functional Interfaces, Karlsruhe Institute of Technology , Hermann-von-Helmholtz-Platz 1, 76344 Eggenstein-Leopoldshafen, Germany.
Inorg Chem. 2017 Mar 20;56(6):3526-3531. doi: 10.1021/acs.inorgchem.6b03140. Epub 2017 Mar 7.
We report a facile approach to prepare metal-nanocatalyst-incorporated carbon thin films with uniform size distribution via carbonization of surface-mounted metal-organic frameworks (SURMOFs) and metal oxo-clusters loaded SURMOF. The calcinated thin films have high performance of methylene blue degradation and the reduction of nitrobenzene. This study describes a general strategy for preparing various nanoparticle-impregnated porous carbon thin films for applications in catalysis.
我们报道了一种简便的方法，通过表面安装的金属有机框架（SURMOFs）和负载金属氧簇的SURMOF碳化来制备尺寸分布均匀的金属纳米催化剂掺入的碳薄膜。煅烧后的薄膜具有高效的亚甲基蓝降解性能和硝基苯还原性能。本研究描述了一种制备各种纳米颗粒浸渍多孔碳薄膜用于催化应用的通用策略。
