Lee Jin-Wook, Hsieh Yao-Tsung, De Marco Nicholas, Bae Sang-Hoon, Han Qifeng, Yang Yang
Department of Materials Science and Engineering and California NanoSystems Institute, University of California , Los Angeles, California 90095, United States.
J Phys Chem Lett. 2017 May 4;8(9):1999-2011. doi: 10.1021/acs.jpclett.7b00374. Epub 2017 Apr 24.
Perovskite solar cells have become one of the strongest candidates for next-generation solar energy technologies. A myriad of beneficial optoelectronic properties of the perovskite materials have enabled superb power conversion efficiencies (PCE) exceeding 22% for a single-junction device. The high PCE achievable via low processing costs and relatively high variability in optical properties have opened new possibilities for perovskites in tandem solar cells. In this Perspective, we will discuss current research trends in fabricating tandem perovskite-based solar cells in combination with a variety of mature photovoltaic devices such as organic, silicon, and Cu(In,Ga)(S,Se) (CIGS) solar cells. Characteristic features and present limitations of each tandem cell will be discussed and elaborated upon. Finally, key issues for further improvement and the future outlook will be discussed.
钙钛矿太阳能电池已成为下一代太阳能技术最有力的候选者之一。钙钛矿材料众多有益的光电特性使单结器件的功率转换效率(PCE)超过22%,表现出色。通过低成本加工可实现的高PCE以及光学性质相对较大的可变性为钙钛矿在串联太阳能电池中开辟了新的可能性。在这篇视角文章中,我们将讨论结合各种成熟的光伏器件(如有机、硅和铜铟镓硒(CIGS)太阳能电池)制造基于钙钛矿的串联太阳能电池的当前研究趋势。将讨论并详细阐述每种串联电池的特征和当前局限性。最后,将讨论进一步改进的关键问题和未来展望。