Department of Physics, University of Seoul, Seoul 02504, Korea.
Nanoscale. 2017 May 11;9(18):6041-6047. doi: 10.1039/c7nr00339k.
Graphene bubbles are often formed when graphene and other layered two-dimensional materials are vertically stacked as van der Waals heterostructures. Here, we investigate how graphene bubbles and their related disorder impact the quantum transport behavior of graphene in the absence and presence of external magnetic fields. By combining experimental observations and numerical simulations, we find that the disorder induced by the graphene bubbles is mainly from p-type dopants and the charge transport in pristine graphene can be severely influenced by the presence of bubbles via long- and short-range scattering even with a small bubble-coverage of 2% and below. Upon bubble density increase, we observe an overall decrease in carrier mobility, and the appearance of a second Dirac point on the electron carrier side. At high magnetic fields, the disorder from graphene bubbles primarily impacts the quantization of the lowest Landau level, resulting in quantum Hall features associated with a new Dirac cone at high charge carrier density.
石墨烯气泡通常在石墨烯和其他层状二维材料作为范德华异质结构垂直堆叠时形成。在这里,我们研究了石墨烯气泡及其相关无序性如何影响没有和存在外磁场时石墨烯的量子输运行为。通过结合实验观察和数值模拟,我们发现,由石墨烯气泡引起的无序主要来自 p 型掺杂剂,并且即使在气泡覆盖率为 2%及以下的情况下,通过长程和短程散射,原始石墨烯中的电荷输运也会受到气泡的严重影响。随着气泡密度的增加,我们观察到载流子迁移率的整体下降,并且在电子载流子侧出现了第二个狄拉克点。在高磁场下,来自石墨烯气泡的无序主要影响最低朗道能级的量子化,导致与高电荷载流密度下的新狄拉克锥相关的量子霍尔特征。