Foundation for Research and Technology-Hellas, Institute of Electronic Structure &Laser, PO Box 1527, GR-71110 Heraklion, Greece.
Department of Physics, University of Crete, 71103 Heraklion, Greece.
Nat Commun. 2017 Apr 27;8:15170. doi: 10.1038/ncomms15170.
High-order harmonics in the extreme-ultraviolet spectral range, resulting from the strong-field laser-atom interaction, have been used in a broad range of fascinating applications in all states of matter. In the majority of these studies the harmonic generation process is described using semi-classical theories which treat the electromagnetic field of the driving laser pulse classically without taking into account its quantum nature. In addition, for the measurement of the generated harmonics, all the experiments require diagnostics in the extreme-ultraviolet spectral region. Here by treating the driving laser field quantum mechanically we reveal the quantum-optical nature of the high-order harmonic generation process by measuring the photon number distribution of the infrared light exiting the harmonic generation medium. It is found that the high-order harmonics are imprinted in the photon number distribution of the infrared light and can be recorded without the need of a spectrometer in the extreme-ultraviolet.
在物质的所有状态中,由于强场激光与原子的相互作用而产生的极紫外光谱范围内的高阶谐波,已经在许多令人着迷的应用中得到了广泛的应用。在这些研究中的大多数中,谐波产生过程是使用半经典理论来描述的,该理论将驱动激光脉冲的电磁场经典地处理,而不考虑其量子性质。此外,对于所产生的谐波的测量,所有的实验都需要在极紫外光谱区域进行诊断。在这里,通过对驱动激光场进行量子力学处理,我们通过测量从谐波产生介质出射的红外光的光子数分布,揭示了高阶谐波产生过程的量子光学性质。结果发现,高阶谐波被印刻在红外光的光子数分布中,并且无需在极紫外光谱区域中使用光谱仪即可记录。