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δ 掺杂 SmTiO 中的非常规电子态。

Unconventional electron states in δ-doped SmTiO.

机构信息

I. Institut für Theoretische Physik, Universität Hamburg, D-20355, Hamburg, Germany.

Institut für Keramische Hochleistungswerkstoffe, Technische Universität Hamburg-Harburg, D-21073, Hamburg, Germany.

出版信息

Sci Rep. 2017 May 8;7(1):1565. doi: 10.1038/s41598-017-01847-5.

Abstract

The Mott-insulating distorted perovskite SmTiO, doped with a single SrO layer in a quantum-well architecture is studied by the combination of density functional theory with dynamical mean-field theory. A rich correlated electronic structure in line with recent experimental investigations is revealed by the given realistic many-body approach to a large-unit-cell oxide heterostructure. Coexistence of conducting and Mott-insulating TiO layers prone to magnetic order gives rise to multi-orbital electronic transport beyond standard Fermi-liquid theory. First hints towards a pseudogap opening due to electron-electron scattering within a background of ferromagnetic and antiferromagnetic fluctuations are detected.

摘要

采用密度泛函理论与动态平均场理论相结合的方法,研究了量子阱结构中掺杂单层 SrO 的扭曲钙钛矿 SmTiO 多晶型体的 Mott 绝缘特性。通过对大型单元氧化物异质结构的实际多体方法的研究,揭示了与近期实验研究相符的丰富关联电子结构。导电和 Mott 绝缘 TiO 层的共存,易产生磁有序,从而导致超出标准费米液体理论的多轨道电子输运。在铁磁和反铁磁涨落的背景下,由于电子-电子散射,检测到了由于赝能隙打开的初步迹象。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/af90/5431486/6f4dfde1023c/41598_2017_1847_Fig1_HTML.jpg

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