Liu Chuanbo, Wang Tianshu, Bai Yawen, Wang Jin
State Key Laboratory of Electroanalytical Chemistry, Changchun Institute of Applied Chemistry, Chinese Academy of Sciences, Changchun, Jilin, P.R. China, 130022.
University of Chinese Academy of Sciences, Beijing, P.R. China, 130022.
PLoS One. 2017 May 26;12(5):e0178405. doi: 10.1371/journal.pone.0178405. eCollection 2017.
A unified picture to understand the protein recognition and function must include the native binding complex structure ensembles and the underlying binding mechanisms involved in specific biological processes. However, quantifications of both binding complex structures and dynamical mechanisms are still challenging for IDP. In this study, we have investigated the underlying molecular mechanism of the chaperone Chz1 and histone H2A.Z-H2B association by equilibrium and kinetic stopped-flow fluorescence spectroscopy. The dependence of free energy and kinetic rate constant on electrolyte mean activity coefficient and urea concentration are uncovered. Our results indicate a previous unseen binding kinetic intermediate. An initial conformation selection step of Chz1 is also revealed before the formation of this intermediate state. Based on these observations, a mixed mechanism of three steps including both conformation selection and induced fit is proposed. By combination of the ion- and denaturant-induced experiments, we demonstrate that electrostatic forces play a dominant role in the recognition of bipolar charged intrinsically disordered protein Chz1 to its preferred partner H2A.Z-H2B. Both the intra-chain and inter-chain electrostatic interactions have direct impacts on the native collapsed structure and binding mechanism.
要理解蛋白质识别与功能,一个统一的图景必须包含天然结合复合物结构集合以及特定生物过程中涉及的潜在结合机制。然而,对于内在无序蛋白(IDP)而言,对结合复合物结构和动力学机制进行量化仍然具有挑战性。在本研究中,我们通过平衡态和动力学停流荧光光谱研究了伴侣蛋白Chz1与组蛋白H2A.Z - H2B结合的潜在分子机制。揭示了自由能和动力学速率常数对电解质平均活度系数和尿素浓度的依赖性。我们的结果表明存在一个之前未被发现的结合动力学中间体。在这个中间体状态形成之前,还揭示了Chz1的一个初始构象选择步骤。基于这些观察结果,提出了一个包括构象选择和诱导契合的三步混合机制。通过结合离子诱导和变性剂诱导实验,我们证明静电力在双极带电的内在无序蛋白Chz1对其偏好伴侣H2A.Z - H2B的识别中起主导作用。链内和链间静电相互作用都对天然折叠结构和结合机制有直接影响。