Department of Chemistry and Biochemistry, Charles E. Schmidt College of Science, Florida Atlantic University, 777 Glades Road, Boca Raton, FL, 33431, USA.
Torrey Pines Institute for Molecular Studies, 11350 SW Village Parkway, Port Saint Lucie, FL, 34987, USA.
Amino Acids. 2017 Nov;49(11):1867-1883. doi: 10.1007/s00726-017-2485-3. Epub 2017 Sep 11.
The transformation from normal to malignant phenotype in human cancers is associated with aberrant cell-surface glycosylation. Thus, targeting glycosylation changes in cancer is likely to provide not only better insight into the roles of carbohydrates in biological systems, but also facilitate the development of new molecular probes for bioanalytical and biomedical applications. In the reported study, we have synthesized lectinomimics based on odorranalectin 1; the smallest lectin-like cyclic peptide isolated from the frog Odorrana grahami skin, and assessed the ability of these peptides to bind specific carbohydrates on molecular and cellular levels. In addition, we have shown that the disulfide bond found in 1 can be replaced with a lactam bridge. However, the orientation of the lactam bridge, peptides 2 and 3, influenced cyclic peptide's conformation and thus these peptides' ability to bind carbohydrates. Naturally occurring 1 and its analog 3 that adopt similar conformation in water bind preferentially L-fucose, and to a lesser degree D-galactose and N-acetyl-D-galactosamine, typically found within the mucin O-glycan core structures. In cell-based assays, peptides 1 and 3 showed a similar binding profile to Aleuria aurantia lectin and these two peptides inhibited the migration of metastatic breast cancer cell lines in a Transwell assay. Altogether, the reported data demonstrate the feasibility of designing lectinomimics based on cyclic peptides.
人类癌症中正常表型向恶性表型的转化与细胞表面糖基化的异常有关。因此,针对癌症中的糖基化变化进行研究,不仅可能提供对碳水化合物在生物系统中作用的更好理解,还可能促进用于生物分析和生物医学应用的新分子探针的开发。在报道的研究中,我们基于气味联觉素 1 合成了凝集素类似物;气味联觉素 1 是从小青蛙 Odorrana grahami 皮肤中分离出来的最小的凝集素样环肽,并评估了这些肽在分子和细胞水平上结合特定碳水化合物的能力。此外,我们已经表明,在 1 中发现的二硫键可以被内酰胺桥取代。然而,内酰胺桥的取向,即肽 2 和 3,影响了环肽的构象,从而影响了这些肽结合碳水化合物的能力。在水中采用相似构象的天然存在的 1 及其类似物 3 优先结合 L-岩藻糖,并且在较小程度上结合 D-半乳糖和 N-乙酰-D-半乳糖胺,这些糖通常存在于粘蛋白 O-聚糖核心结构中。在基于细胞的测定中,肽 1 和 3 与 Aleuria aurantia 凝集素表现出相似的结合模式,并且这两种肽在 Transwell 测定中抑制转移性乳腺癌细胞系的迁移。总之,报道的数据表明基于环肽设计凝集素类似物是可行的。