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三层镍酸盐LaNiO的费米学与电子动力学

Fermiology and electron dynamics of trilayer nickelate LaNiO.

作者信息

Li Haoxiang, Zhou Xiaoqing, Nummy Thomas, Zhang Junjie, Pardo Victor, Pickett Warren E, Mitchell J F, Dessau D S

机构信息

Department of Physics, University of Colorado at Boulder, Boulder, CO, 80309, USA.

Material Science Division, Argonne National Lab, Argonne, IL, 60439, USA.

出版信息

Nat Commun. 2017 Sep 26;8(1):704. doi: 10.1038/s41467-017-00777-0.

Abstract

Layered nickelates have the potential for exotic physics similar to high T superconducting cuprates as they have similar crystal structures and these transition metals are neighbors in the periodic table. Here we present an angle-resolved photoemission spectroscopy (ARPES) study of the trilayer nickelate LaNiO revealing its electronic structure and correlations, finding strong resemblances to the cuprates as well as a few key differences. We find a large hole Fermi surface that closely resembles the Fermi surface of optimally hole-doped cuprates, including its [Formula: see text] orbital character, hole filling level, and strength of electronic correlations. However, in contrast to cuprates, LaNiO has no pseudogap in the [Formula: see text] band, while it has an extra band of principally [Formula: see text] orbital character, which presents a low temperature energy gap. These aspects drive the nickelate physics, with the differences from the cuprate electronic structure potentially shedding light on the origin of superconductivity in the cuprates.Exploration of the electronic structure of nickelates with similar crystal structure to cuprates may shed a light on the origin of high T superconductivity. Here, Li et al. report strong resemblances and key differences of the electronic structure of trilayer nickelate LaNiO compared to the cuprate superconductors.

摘要

层状镍酸盐具有与高温超导铜酸盐类似的奇异物理特性的潜力,因为它们具有相似的晶体结构,且这些过渡金属在元素周期表中相邻。在此,我们展示了一项对三层镍酸盐LaNiO进行的角分辨光电子能谱(ARPES)研究,揭示了其电子结构和相关性,发现它与铜酸盐有很强的相似性以及一些关键差异。我们发现一个大的空穴费米面,它与最佳空穴掺杂铜酸盐的费米面非常相似,包括其[公式:见正文]轨道特征、空穴填充水平和电子相关性强度。然而,与铜酸盐不同的是,LaNiO在[公式:见正文]能带中没有赝能隙,而它有一个主要具有[公式:见正文]轨道特征的额外能带,呈现出一个低温能隙。这些方面推动了镍酸盐的物理特性,与铜酸盐电子结构的差异可能为铜酸盐中超导性的起源提供线索。对具有与铜酸盐相似晶体结构的镍酸盐电子结构的探索可能会为高温超导的起源提供线索。在此,Li等人报告了三层镍酸盐LaNiO与铜酸盐超导体相比,其电子结构的强烈相似性和关键差异。

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