Laboratoire de Physique des Solides, Université Paris-Sud, UMR 8502, Bâtiment 510, 91405 Orsay, France.
Phys Rev Lett. 2013 Apr 19;110(16):167002. doi: 10.1103/PhysRevLett.110.167002. Epub 2013 Apr 16.
Using angle-resolved photoemission spectroscopy, we study the evolution of the number of carriers in Ba(Fe(1-x)Co(x))(2)As(2) as a function of Co content and temperature. We show that there is a k-dependent energy shift compared to density functional calculations, which is large below 100 K at low Co contents and reduces the volume of hole and electron pockets by a factor 2. This k shift becomes negligible at high Co content and could be due to interband charge or spin fluctuations. We further reveal that the bands shift with temperature, changing significantly the number of carriers they contain (up to 50%). We explain this evolution by thermal excitations of carriers among the narrow bands, possibly combined with a temperature evolution of the k-dependent fluctuations.
我们使用角分辨光电子能谱研究 Ba(Fe(1-x)Co(x))(2)As(2)中载流子数量随 Co 含量和温度的变化。我们表明,与密度泛函计算相比,存在与 k 相关的能量位移,在低 Co 含量下低于 100 K 时较大,并将空穴和电子口袋的体积减小了 2 倍。在高 Co 含量下,这种 k 位移变得可以忽略不计,可能是由于带间电荷或自旋涨落。我们进一步揭示,能带随温度变化,这会显著改变它们所包含的载流子数量(高达 50%)。我们通过窄带中载流子的热激发来解释这种演变,可能与 k 相关涨落的温度演化相结合。