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双层支石墓阵列纳米结构中的圆二色性效应

Circular dichroism effect in a double-layer dolmen array nanostructure.

作者信息

Liu Youyao, Yu Xiaoshan

出版信息

Appl Opt. 2017 Aug 1;56(22):6263-6266. doi: 10.1364/AO.56.006263.

Abstract

Chiral plasmonic nanostructures have been studied widely in past years and have various applications in biological sensing, negative refractive indexing, and analytical chemistry. Dolmen is also a commonly used nanostructure in many recent research papers. By placing dolmens in different directions and forming a double-layer dolmen array (DLDA), a new nanostructure with good circular dichroism (CD) effect is designed in this paper. We get up to the maximum of 0.5 of CD effect through numerical simulation. Among three obvious resonance wavelengths of CD effect, magnetic dipole resonance appears in two of them and contributes to the origin of a strong CD effect. In these different coupling modes, the strongest one locating at the largest wavelength is the result of a big magnetic dipolar resonance generated by circulation current in two layers of dolmen together, and the second strongest CD effect is caused by individual magnetic dipolar resonance in the opposite direction located in each layer. At the weakest one, the circulation current disappears and only a regular electric dipolar resonance appears. This simulation result shows that magnetic dipolar resonance of plasmonic nanostructure could create a strong CD effect, and much more effectively in the DLDA we propose. The results can help us in designing novel chiral optical nanostructures and provide applications in the interactions between photons and electrons.

摘要

近年来,手性等离子体纳米结构得到了广泛研究,并在生物传感、负折射率和分析化学等领域有多种应用。多尔门也是许多近期研究论文中常用的纳米结构。通过将多尔门放置在不同方向并形成双层多尔门阵列(DLDA),本文设计了一种具有良好圆二色性(CD)效应的新型纳米结构。通过数值模拟,我们得到了高达0.5的CD效应最大值。在CD效应的三个明显共振波长中,其中两个出现磁偶极共振,这有助于产生强烈的CD效应。在这些不同的耦合模式中,位于最大波长处最强的耦合模式是由两层多尔门中的环流产生的大磁偶极共振的结果,第二强的CD效应是由每层中相反方向的单个磁偶极共振引起的。在最弱的耦合模式下,环流消失,只出现规则的电偶极共振。该模拟结果表明,等离子体纳米结构的磁偶极共振可以产生强烈的CD效应,并且在我们提出的DLDA中更有效。这些结果有助于我们设计新型手性光学纳米结构,并为光子与电子之间的相互作用提供应用。

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