a Department of Medicinal Chemistry , L. S. Skaggs Pharmacy Institute, University of Utah , Salt Lake City , UT 84112 , USA.
J Biomol Struct Dyn. 2018 Oct;36(13):3311-3323. doi: 10.1080/07391102.2017.1389306. Epub 2017 Nov 3.
The catechin family of molecules that are present in the leaves of green tea has been under investigation since the antioxidant and anti-inflammatory properties of tea were discovered. Among multiple proposed therapeutic targets of these molecules, the direct interaction with nucleic acids has been proposed and experimentally observed but without clear knowledge about the potential binding modes between these ligands and DNA. One of these catechin structures, (-)-epigallocatechin gallate (EGCG), has three aromatic rings that could interact with double-stranded DNA via terminal base-pair stacking, intercalation, or through groove binding. Using enhanced sampling techniques and molecular dynamics simulations, we have found a stable complex between the EGCG ligand and DNA through intercalation of the trihydroxybenzoate aromatic ring and an ApC step. Moreover, we have calculated the absorption spectra of four possible binding modes and compared these to absorption profiles reported in the literature, and explored the possible DNA sequence preference for the EGCG ligand to bind. Our results suggest that an intercalative mode of interaction through the major groove is possible between the EGCG ligands and DNA with apparently very little DNA sequence selectivity.
儿茶素家族的分子存在于绿茶的叶子中,自从发现茶的抗氧化和抗炎特性以来,一直受到研究。在这些分子的多个提出的治疗靶点中,已经提出并实验观察到它们与核酸的直接相互作用,但对于这些配体与 DNA 之间的潜在结合模式知之甚少。儿茶素结构之一,(-)-表没食子儿茶素没食子酸酯(EGCG),有三个芳环,可以通过末端碱基对堆积、嵌入或通过沟结合与双链 DNA 相互作用。使用增强采样技术和分子动力学模拟,我们通过三羟基苯甲酸芳环的嵌入和 ApC 步找到了 EGCG 配体与 DNA 之间的稳定复合物。此外,我们计算了四种可能的结合模式的吸收光谱,并将其与文献中报道的吸收谱进行了比较,还探讨了 EGCG 配体结合的可能 DNA 序列偏好。我们的结果表明,EGCG 配体与 DNA 之间可能通过主槽发生嵌入相互作用,并且 DNA 序列选择性很小。