Talbo Vincent, Saint-Martin Jérôme, Retailleau Sylvie, Dollfus Philippe
Univ. Grenoble Alpes, CEA, INAC-Pheliqs, 38000, Grenoble, France.
Centre de Nanosciences et de Nanotechnologies, CNRS, Univ. Paris-Sud, Université Paris-Saclay, C2N - Orsay, 91405, Orsay, cedex, France.
Sci Rep. 2017 Nov 1;7(1):14783. doi: 10.1038/s41598-017-14009-4.
By means of advanced numerical simulation, the thermoelectric properties of a Si-quantum dot-based single-electron transistor operating in sequential tunneling regime are investigated in terms of figure of merit, efficiency and power. By taking into account the phonon-induced collisional broadening of energy levels in the quantum dot, both heat and electrical currents are computed in a voltage range beyond the linear response. Using our homemade code consisting in a 3D Poisson-Schrödinger solver and the resolution of the Master equation, the Seebeck coefficient at low bias voltage appears to be material independent and nearly independent on the level broadening, which makes this device promising for metrology applications as a nanoscale standard of Seebeck coefficient. Besides, at higher voltage bias, the non-linear characteristics of the heat current are shown to be related to the multi-level effects. Finally, when considering only the electronic contribution to the thermal conductance, the single-electron transistor operating in generator regime is shown to exhibit very good efficiency at maximum power.
通过先进的数值模拟,从优值、效率和功率方面研究了处于顺序隧穿 regime 下的基于硅量子点的单电子晶体管的热电特性。考虑到量子点中声子诱导的能级碰撞展宽,在超出线性响应的电压范围内计算了热电流和电电流。使用我们自制的包含三维泊松 - 薛定谔求解器和主方程求解的代码,低偏置电压下的塞贝克系数似乎与材料无关且几乎与能级展宽无关,这使得该器件作为塞贝克系数的纳米级标准在计量应用中具有前景。此外,在较高电压偏置下,热电流的非线性特性被证明与多能级效应有关。最后,当仅考虑电子对热导率的贡献时,处于发电机 regime 下工作的单电子晶体管在最大功率下表现出非常好的效率。