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河流中人为合成与非合成纤维:采样方法学方面及通量估算,受巴黎大都市影响。

Synthetic and non-synthetic anthropogenic fibers in a river under the impact of Paris Megacity: Sampling methodological aspects and flux estimations.

机构信息

Université Paris-Est, Laboratoire Eau, Environnement, Systèmes Urbains (LEESU), UMR MA 102 - AgroParisTech, 61 Avenue du Général de Gaulle, Créteil Cedex, France.

Université Paris-Est, Laboratoire Eau, Environnement, Systèmes Urbains (LEESU), UMR MA 102 - AgroParisTech, 61 Avenue du Général de Gaulle, Créteil Cedex, France.

出版信息

Sci Total Environ. 2018 Mar 15;618:157-164. doi: 10.1016/j.scitotenv.2017.11.009. Epub 2017 Nov 9.

DOI:10.1016/j.scitotenv.2017.11.009
PMID:29128764
Abstract

Processed fibers are highly present in our daily life and can be either natural, artificial (regenerated cellulose) and synthetic (made with petrochemicals). Their widespread use lead inevitably to a high contamination of environment. Previous studies focus on plastic particles regardless of their type or shape as long as they are comprised between 330μm and 5mm. On the contrary, this study focuses exclusively on fibers using a smaller mesh size net (80μm) to sample freshwater. Moreover, all processed organic fibers are considered, irrespective to their nature. First, the short term temporal variability of the fibers in the environment was assessed. While exposing the sampling net during 1min a coefficient of variation of approx. 45% (with n=6) was determined. It was of only 26% (n=6) when the exposure was of 3min. The assessment of the distribution through the section showed a possible difference in concentrations between the middle of the water surface and the river banks which could be attributed to the intense river traffic within the Paris Megacity. The vertical variability seems negligible as turbulence and current conditions homogenize the distribution of the fibers. A monthly monitoring showed concentrations of 100.6±99.9fibers·m in the Marne River and of: 48.5±98.5, 27.9±26.3, 27.9±40.3 and 22.1±25.3fibers·m from the upstream to downstream points in the Seine River. Once these concentrations are converted into fluxes, it seems that the impact generated by the Paris Megacity cannot be distinguished. Investigations on the role of sedimentation and deposition on the banks are required. This study helped fill some major knowledge gaps regarding the fibers in rivers, their sampling, occurrence, spatial-temporal distribution and fluxes. It is encouraged that future studies include both synthetic and none synthetic fibers.

摘要

加工纤维在我们的日常生活中大量存在,它们可以是天然的、人工的(再生纤维素)和合成的(由石化产品制成)。由于它们的广泛使用,不可避免地导致了环境的高度污染。以前的研究主要集中在塑料颗粒上,而不管它们的类型或形状,只要它们在 330μm 和 5mm 之间。相比之下,本研究仅专注于使用较小网眼尺寸的网(80μm)来采集淡水的纤维。此外,所有加工有机纤维都被考虑在内,而不论其性质如何。首先,评估了环境中纤维的短期时间变化性。当暴露采样网 1 分钟时,确定了约 45%(n=6)的变异系数。当暴露时间为 3 分钟时,变异系数仅为 26%(n=6)。通过截面评估分布情况,发现水面中部和河岸之间的浓度可能存在差异,这可能归因于巴黎大都市内密集的河流交通。垂直变化似乎可以忽略不计,因为湍流和水流条件使纤维的分布均匀化。每月监测显示,在马恩河中的浓度为 100.6±99.9 根纤维·m,而在塞纳河从上游到下游的各个点的浓度分别为:48.5±98.5、27.9±26.3、27.9±40.3 和 22.1±25.3 根纤维·m。一旦将这些浓度转换为通量,似乎就无法区分巴黎大都市产生的影响。需要对沉积和沉积在河岸上的作用进行调查。本研究有助于填补有关河流中纤维、采样、出现、时空分布和通量的一些主要知识空白。鼓励未来的研究包括合成纤维和非合成纤维。

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