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LiF:Mg,Ti(哈肖)热释光中剂量率效应的综述

REVIEW OF DOSE-RATE EFFECTS IN THE THERMOLUMINESCENCE OF Lif:mg,ti (HARSHAW).

作者信息

Horowitz Yigal, Oster Leonid, Eliyahu Ilan

机构信息

Physics Department, Ben Gurion University of the Negev, Beersheva, Israel.

Physics Unit, Sami Shamoon College of Engineering, Beersheva, Israel.

出版信息

Radiat Prot Dosimetry. 2018 Apr 1;179(2):184-188. doi: 10.1093/rpd/ncx248.

Abstract

The literature describing the experimental investigations of possible dose-rate effects in the thermoluminescence (TL) of LiF:Mg,Ti (Harshaw) is reviewed. The total lack of glow curve analysis, coupled with inclusion of all or part of the high temperature TL and absence of parallel measurements of possible dose-rate effects in the irradiation stage severely limit the scientific and technical level of the experiments. In addition, the experimental procedures are far from sufficient to warrant any conclusion concerning the presence or absence of dose-rate effects in the TL of LiF:Mg,Ti. This decision is contrary to the widely held belief that there are no dose-rate effects in the TL of LiF:Mg,Ti. In addition, the literature on dose-rate effects in the optical absorption (irradiation stage) of LiF is reviewed and is found contradictory. No dose-rate studies have been carried out on optical absorption in LiF:Mg,Ti. Kinetic simulations demonstrating the possibility, even likelihood, of dose-rate effects are also reviewed. Dose-rate effects are shown to be likely due to competition between excitation and recombination in the irradiation stage. Some other possible mechanisms involving multiple charge carrier trapping are suggested. Further definitive experiments are sorely needed, but the interested researcher should beware, it is not an easy task.

摘要

回顾了描述对LiF:Mg,Ti(哈肖)热释光(TL)中可能存在的剂量率效应进行实验研究的文献。完全缺乏发光曲线分析,再加上纳入了全部或部分高温热释光,并且在辐照阶段没有对可能的剂量率效应进行平行测量,这严重限制了实验的科学技术水平。此外,实验程序远远不足以支持就LiF:Mg,Ti热释光中是否存在剂量率效应得出任何结论。这一结论与普遍认为LiF:Mg,Ti热释光中不存在剂量率效应的观点相反。此外,还回顾了关于LiF光吸收(辐照阶段)中剂量率效应的文献,发现其相互矛盾。尚未对LiF:Mg,Ti中的光吸收进行剂量率研究。还回顾了动力学模拟,这些模拟证明了剂量率效应存在的可能性,甚至是可能性很大。结果表明,剂量率效应可能是由于辐照阶段激发与复合之间的竞争所致。还提出了一些涉及多电荷载流子俘获的其他可能机制。迫切需要进一步的确定性实验,但感兴趣的研究人员应该注意,这并非易事。

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