• 文献检索
  • 文档翻译
  • 深度研究
  • 学术资讯
  • Suppr Zotero 插件Zotero 插件
  • 邀请有礼
  • 套餐&价格
  • 历史记录
应用&插件
Suppr Zotero 插件Zotero 插件浏览器插件Mac 客户端Windows 客户端微信小程序
定价
高级版会员购买积分包购买API积分包
服务
文献检索文档翻译深度研究API 文档MCP 服务
关于我们
关于 Suppr公司介绍联系我们用户协议隐私条款
关注我们

Suppr 超能文献

核心技术专利:CN118964589B侵权必究
粤ICP备2023148730 号-1Suppr @ 2026

文献检索

告别复杂PubMed语法,用中文像聊天一样搜索,搜遍4000万医学文献。AI智能推荐,让科研检索更轻松。

立即免费搜索

文件翻译

保留排版,准确专业,支持PDF/Word/PPT等文件格式,支持 12+语言互译。

免费翻译文档

深度研究

AI帮你快速写综述,25分钟生成高质量综述,智能提取关键信息,辅助科研写作。

立即免费体验

光致激子有序增强

Photoinduced Enhancement of Excitonic Order.

作者信息

Murakami Yuta, Golež Denis, Eckstein Martin, Werner Philipp

机构信息

Department of Physics, University of Fribourg, 1700 Fribourg, Switzerland.

Department of Physics, University of Erlangen-Nürnberg, 91058 Erlangen, Germany.

出版信息

Phys Rev Lett. 2017 Dec 15;119(24):247601. doi: 10.1103/PhysRevLett.119.247601.

DOI:10.1103/PhysRevLett.119.247601
PMID:29286755
Abstract

We study the dynamics of excitonic insulators coupled to phonons using the time-dependent mean-field theory. Without phonon couplings, the linear response is given by the damped amplitude oscillations of the order parameter with a frequency equal to the minimum band gap. A phonon coupling to the interband transfer integral induces two types of long-lived collective oscillations of the amplitude, one originating from the phonon dynamics and the other from the phase mode, which becomes massive. We show that, even for small phonon coupling, a photoinduced enhancement of the exciton condensation and the gap can be realized. Using the Anderson pseudospin picture, we argue that the origin of the enhancement is a cooperative effect of the massive phase mode and the Hartree shift induced by the photoexcitation. We also discuss how the enhancement of the order and the collective modes can be observed with time-resolved photoemission spectroscopy.

摘要

我们使用含时平均场理论研究了与声子耦合的激子绝缘体的动力学。在没有声子耦合的情况下,线性响应由序参量的阻尼振幅振荡给出,其频率等于最小带隙。声子与带间转移积分的耦合会引发两种长寿命的振幅集体振荡,一种源于声子动力学,另一种源于变为有质量的相位模式。我们表明,即使对于小的声子耦合,也可以实现光致激子凝聚和能隙的增强。利用安德森赝自旋图像,我们认为增强的起源是有质量的相位模式和光激发诱导的哈特里位移的协同效应。我们还讨论了如何通过时间分辨光电子能谱观察序参量和集体模式的增强。

相似文献

1
Photoinduced Enhancement of Excitonic Order.光致激子有序增强
Phys Rev Lett. 2017 Dec 15;119(24):247601. doi: 10.1103/PhysRevLett.119.247601.
2
Multiple coherent amplitude modes and exciton-phonon coupling in quasi-one-dimensional excitonic insulator TaNiSe.准一维激子绝缘体TaNiSe中的多个相干振幅模式与激子-声子耦合
Phys Chem Chem Phys. 2024 May 29;26(21):15417-15425. doi: 10.1039/d4cp00261j.
3
Nonlinear Spectroscopy of Collective Modes in an Excitonic Insulator.激子绝缘体中集体模式的非线性光谱学
Phys Rev Lett. 2020 Dec 18;125(25):257601. doi: 10.1103/PhysRevLett.125.257601.
4
Exciton-phonon system on a star graph: A perturbative approach.星型图上的激子-声子系统:一种微扰方法。
Phys Rev E. 2016 May;93(5):052306. doi: 10.1103/PhysRevE.93.052306. Epub 2016 May 9.
5
Coherent order parameter oscillations in the ground state of the excitonic insulator TaNiSe.激子绝缘体TaNiSe基态中的相干序参量振荡。
Sci Adv. 2018 Mar 23;4(3):eaap8652. doi: 10.1126/sciadv.aap8652. eCollection 2018 Mar.
6
Vibronic enhancement of excitation energy transport: Interplay between local and non-local exciton-phonon interactions.振子能量传递的协同增强:局域激子-声子相互作用与非局域激子-声子相互作用的相互作用。
J Chem Phys. 2017 Feb 21;146(7):075101. doi: 10.1063/1.4976558.
7
Slave rotor approach to exciton condensation in a two-band system.两能带系统中激子凝聚的从属转子方法。
J Phys Condens Matter. 2019 Jan 9;31(1):015601. doi: 10.1088/1361-648X/aaee06. Epub 2018 Nov 30.
8
Room-Temperature Coherent Optical Phonon in 2D Electronic Spectra of CHNHPbI Perovskite as a Possible Cooling Bottleneck.CHNHPbI钙钛矿二维电子光谱中的室温相干光学声子作为可能的冷却瓶颈
J Phys Chem Lett. 2017 Jul 20;8(14):3211-3215. doi: 10.1021/acs.jpclett.7b01357. Epub 2017 Jun 30.
9
The effect of n- and p-type doping on coherent phonons in GaN.n 型和 p 型掺杂对 GaN 中相干声子的影响。
J Phys Condens Matter. 2013 May 22;25(20):205404. doi: 10.1088/0953-8984/25/20/205404. Epub 2013 Apr 25.
10
Exciton-Phonon Interactions in Monolayer Germanium Selenide from First Principles.基于第一性原理的单层硒化锗中的激子 - 声子相互作用
J Phys Chem Lett. 2021 Apr 22;12(15):3802-3808. doi: 10.1021/acs.jpclett.1c00264. Epub 2021 Apr 13.

引用本文的文献

1
The spontaneous symmetry breaking in TaNiSe is structural in nature.TaNiSe 中的自发对称破缺在本质上是结构上的。
Proc Natl Acad Sci U S A. 2023 Apr 25;120(17):e2221688120. doi: 10.1073/pnas.2221688120. Epub 2023 Apr 18.
2
Imaging the coherent propagation of collective modes in the excitonic insulator TaNiSe at room temperature.在室温下对激子绝缘体TaNiSe中集体模式的相干传播进行成像。
Sci Adv. 2021 Jul 7;7(28). doi: 10.1126/sciadv.abd6147. Print 2021 Jul.
3
Light-induced evaporative cooling of holes in the Hubbard model.哈伯德模型中孔洞的光致蒸发冷却
Nat Commun. 2019 Dec 5;10(1):5556. doi: 10.1038/s41467-019-13557-9.
4
Theory of photoinduced ultrafast switching to a spin-orbital ordered hidden phase.光诱导超快相变到自旋轨道有序的隐藏相的理论。
Nat Commun. 2018 Nov 2;9(1):4581. doi: 10.1038/s41467-018-07051-x.
5
Coherent order parameter oscillations in the ground state of the excitonic insulator TaNiSe.激子绝缘体TaNiSe基态中的相干序参量振荡。
Sci Adv. 2018 Mar 23;4(3):eaap8652. doi: 10.1126/sciadv.aap8652. eCollection 2018 Mar.