Chitra N, Danalakshmi B, Supriya D, Vijayalakshmi I, Sundar S Bala, Sivasubramanian K, Baskaran R, Jose M T
Radiological Safety Division, Indira Gandhi Center for Atomic Research, Tamilnadu, India; Homi Bhabha National Institute, Kalpakkam 603102, Tamilnadu, India.
Radiological Safety Division, Indira Gandhi Center for Atomic Research, Tamilnadu, India.
Appl Radiat Isot. 2018 Mar;133:75-80. doi: 10.1016/j.apradiso.2017.12.017. Epub 2017 Dec 19.
The exhalation of radon (Rn) and thoron (Rn) from a porous matrix depends on the emanation of them from the grains by the recoil effect. The emanation factor is a quantitative estimate of the emanation phenomenon. The present study is to investigate the effect of grain size of the soil matrix on the emanation factor. Soil samples from three different locations were fractionated into different grain size categories ranging from <0.1 to 2mm. The emanation factors of each of the grain size range were estimated by measuring the mass exhalation rates of radon and thoron and the activity concentrations of Ra and Th. The emanation factor was found to increase with decrease in grain size. This effect was made evident by keeping the parent radium concentration constant for all grain size fractions. The governing factor is the specific surface area of the soil samples which increases with decrease in grain size.
多孔介质中氡(Rn)和钍射气(Rn)的析出取决于它们通过反冲效应从颗粒中的逸出。逸出系数是对逸出现象的定量估计。本研究旨在调查土壤介质颗粒大小对逸出系数的影响。来自三个不同地点的土壤样本被分成不同的颗粒大小类别,范围从<0.1毫米到2毫米。通过测量氡和钍射气的质量析出率以及镭和钍的活度浓度,估算了每个颗粒大小范围的逸出系数。结果发现,逸出系数随颗粒大小的减小而增加。通过保持所有颗粒大小级分的母体镭浓度恒定,这一效应变得明显。控制因素是土壤样本的比表面积,它随颗粒大小的减小而增加。