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具有反钙钛矿结构的受挫磁体系统中的绝热冷却过程。

Adiabatic cooling processes in frustrated magnetic systems with pyrochlore structure.

机构信息

Institute of Experimental Physics, Slovak Academy of Sciences, Watsonova 47, 040 01 Košice, Slovakia.

Department of Theoretical Physics and Astrophysics, Faculty of Science, P.J. Šafárik University, Park Angelinum 9, 040 01 Košice, Slovakia.

出版信息

Phys Rev E. 2017 Nov;96(5-1):052128. doi: 10.1103/PhysRevE.96.052128. Epub 2017 Nov 20.

Abstract

We investigate in detail the process of adiabatic cooling in the framework of the exactly solvable antiferromagnetic spin-1/2 Ising model in the presence of the external magnetic field on an approximate lattice with pyrochlore structure. The behavior of the entropy of the model is studied and exact values of the residual entropies of all ground states are found. The temperature variation of the system under adiabatic (de)magnetization is investigated and the central role of the macroscopically degenerated ground states in cooling processes is explicitly demonstrated. It is shown that the model parameter space of the studied geometrically frustrated system is divided into five disjunct regions with qualitatively different processes of the adiabatic cooling. The effectiveness of the adiabatic (de)magnetization cooling in the studied model is compared to the corresponding processes in paramagnetic salts. It is shown that the processes of the adiabatic cooling in the antiferromagnetic frustrated systems are much more effective especially in nonzero external magnetic fields. It means that the frustrated magnetic materials with pyrochlore structure can be considered as very promising refrigerants mainly in the situations with nonzero final values of the magnetic field.

摘要

我们在存在外磁场的情况下,详细研究了在准萤石结构近似晶格上,可精确求解的反铁磁自旋-1/2 Ising 模型中的绝热冷却过程。我们研究了模型熵的行为,并找到了所有基态剩余熵的精确值。我们还研究了系统在绝热(去)磁化过程中的温度变化,并明确证明了宏观简并基态在冷却过程中起核心作用。结果表明,所研究的几何受挫系统的模型参数空间被划分为五个不相交的区域,这些区域中存在着绝热冷却的定性不同的过程。我们还将研究模型中的绝热(去)磁化冷却的有效性与顺磁盐中的对应过程进行了比较。结果表明,反铁磁受挫系统中的绝热冷却过程效率更高,特别是在非零外磁场的情况下。这意味着具有萤石结构的受挫磁体材料可被视为很有前途的制冷剂,主要适用于磁场的最终值不为零的情况。

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