He Ju, Wang Shuai, Chen Jingwen, Wu Feng, Dai Jiangnan, Long Hanling, Zhang Yi, Zhang Wei, Feng Zhe Chuan, Zhang Jun, Du Shida, Ye Lei, Chen Changqing
Wuhan National Laboratory for Optoelectronics, Huazhong University of Science and Technology, People's Republic of China.
Nanotechnology. 2018 May 11;29(19):195203. doi: 10.1088/1361-6528/aab168. Epub 2018 Feb 22.
In this paper, we report a 2.6-fold deep ultraviolet emission enhancement of integrated photoluminescence (PL) intensity in AlGaN-based multi-quantum wells (MQWs) by introducing the coupling of local surface plasmons from Al nanoparticles (NPs) on a SiO dielectric interlayer with excitons and photons in MQWs at room temperature. In comparison to bare AlGaN MQWs, a significant 2.3-fold enhancement of the internal quantum efficiency, from 16% to 37%, as well as a 13% enhancement of photon extraction efficiency have been observed in the MQWs decorated with Al NPs on SiO dielectric interlayer. Polarization-dependent PL measurement showed that both the transverse electric and transverse magnetic mode were stronger than the original intensity in bare AlGaN MQWs, indicating a strong LSPs coupling process and vigorous scattering ability of the Al/SiO composite structure. These results were confirmed by the activation energy of non-radiative recombination from temperature-dependent PL measurement and the theoretical three dimensional finite difference time domain calculations.
在本文中,我们报道了通过在室温下引入SiO介电层上Al纳米颗粒(NPs)的局域表面等离子体与多量子阱(MQWs)中的激子和光子的耦合,基于AlGaN的多量子阱(MQWs)的集成光致发光(PL)强度实现了2.6倍的深紫外发射增强。与裸AlGaN多量子阱相比,在SiO介电层上装饰有Al NPs的多量子阱中,内部量子效率显著提高了2.3倍,从16%提高到37%,并且光子提取效率提高了13%。偏振相关的PL测量表明,横向电场和横向磁场模式都比裸AlGaN多量子阱中的原始强度更强,这表明Al/SiO复合结构具有很强的局域表面等离子体耦合过程和强烈的散射能力。通过温度相关PL测量的非辐射复合激活能以及理论三维有限差分时域计算证实了这些结果。