Dept. of Electronics, Carleton University, 1125 Colonel By Dr, Ottawa, ON, Canada.
Nanoscale. 2018 Mar 29;10(13):5914-5922. doi: 10.1039/c7nr09183d.
Single-mode surface plasmon distributed feedback (DFB) lasers are realized in the near infrared using a two-dimensional non-uniform long-range surface plasmon polariton structure. The surface plasmon mode is excited onto a 20 nm-thick, 1 μm-wide metal stripe (Ag or Au) on a silica substrate, where the stripe is stepped in width periodically, forming a 1st order Bragg grating. Optical gain is provided by optically pumping a 450 nm-thick IR-140 doped PMMA layer as the top cladding, which covers the entire length of the Bragg grating, thus creating a DFB laser. Single-mode lasing peaks of very narrow linewidth were observed for Ag and Au DFBs near 882 nm at room temperature. The narrow linewidths are explained by the low spontaneous emission rate into the surface plasmon lasing mode as well as the high quality factor of the DFB structure. The lasing emission is exclusively TM polarized. Kinks in light-light curves accompanied by spectrum narrowing were observed, from which threshold pump power densities can be clearly identified (0.78 MW cm-2 and 1.04 MW cm-2 for Ag and Au DFB lasers, respectively). The Schawlow-Townes linewidth for our Ag and Au DFB lasers is estimated and very narrow linewidths are predicted for the lasers. The lasers are suitable as inexpensive, recyclable and highly coherent sources of surface plasmons, or for integration with other surface plasmon elements of similar structure.
使用二维非均匀长程表面等离子体激元(LRSPP)结构,在近红外实现了单模表面等离子体分布式反馈(DFB)激光器。将表面等离子体模式激励到厚度为 20nm、宽度为 1μm 的金属条(Ag 或 Au)上,其中条带周期性地变宽,形成一阶布拉格光栅。通过对覆盖布拉格光栅全长的 450nm 厚掺 IR-140 的 PMMA 层进行光泵浦来提供光学增益,从而创建 DFB 激光器。在室温下,Ag 和 Au DFB 在 882nm 附近观察到非常窄线宽的单模激光峰。窄线宽可以通过将自发发射率降低到表面等离子体激光模式以及 DFB 结构的高品质因数来解释。激光发射是完全 TM 偏振的。观察到伴随着光谱变窄的光-光曲线中的拐点,可以清楚地识别出阈值泵浦功率密度(Ag 和 Au DFB 激光器分别为 0.78MWcm-2 和 1.04MWcm-2)。我们的 Ag 和 Au DFB 激光器的肖洛-汤斯线宽进行了估计,并预测了非常窄的线宽。这些激光器适合作为低成本、可回收和高度相干的表面等离子体源,或与具有类似结构的其他表面等离子体元件集成。