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亚洲水塔河流中溶解的碳质和氮质物质的输出。

Export of dissolved carbonaceous and nitrogenous substances in rivers of the "Water Tower of Asia".

机构信息

Laboratory of Green Chemistry, Lappeenranta University of Technology, Mikkeli 50130, Finland.

Laboratory of Green Chemistry, Lappeenranta University of Technology, Mikkeli 50130, Finland.

出版信息

J Environ Sci (China). 2018 Mar;65:53-61. doi: 10.1016/j.jes.2017.04.001. Epub 2017 Apr 8.

Abstract

Rivers are critical links in the carbon and nitrogen cycle in aquatic, terrestrial, and atmospheric environments. Here riverine carbon and nitrogen exports in nine large rivers on the Tibetan Plateau - the "Water Tower of Asia" - were investigated in the monsoon season from 2013 to 2015. Compared with the world average, concentrations of dissolved inorganic carbon (DIC, 30.7mg/L) were high in river basins of the plateau due to extensive topographic relief and intensive water erosion. Low concentrations of dissolved organic carbon (DOC, 1.16mg/L) were likely due to the low temperature and unproductive land vegetation environments. Average concentrations of riverine DIN (0.32mg/L) and DON (0.35 mg/L) on the Tibetan Plateau were close to the world average. However, despite its predominantly pristine environment, discharge from agricultural activities and urban areas of the plateau has raised riverine N export. In addition, DOC/DON ratio (C/N, ~6.5) in rivers of the Tibetan Plateau was much lower than the global average, indicating that dissolved organic carbon in the rivers of this region might be more bioavailable. Therefore, along with global warming and anthropogenic activities, increasing export of bioavailable riverine carbon and nitrogen from rivers of the Tibetan Plateau can be expected in the future, which will possibly influence the regional carbon and nitrogen cycle.

摘要

河流是水生、陆地和大气环境中碳氮循环的关键环节。本研究于 2013 年至 2015 年季风季节调查了亚洲水塔——青藏高原九大河流的河川碳氮输出。与世界平均值相比,由于高原地区广泛的地形抬升和强烈的水力侵蚀,流域中溶解无机碳(DIC,30.7mg/L)的浓度较高。由于低温和贫瘠的陆地植被环境,溶解有机碳(DOC,1.16mg/L)的浓度可能较低。高原河流水体 DIN(0.32mg/L)和 DON(0.35mg/L)的平均浓度接近世界平均值。然而,尽管青藏高原环境基本原始,但来自农业活动和高原城区的排放增加了河川氮素的输出。此外,青藏高原河流的 DOC/DON 比值(C/N,~6.5)远低于全球平均值,表明该地区河流中的溶解有机碳可能更具生物可利用性。因此,随着全球变暖及人为活动的影响,未来青藏高原河流中生物可利用的河川碳氮输出预计会增加,这可能会影响区域碳氮循环。

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