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创新褐煤活性炭辅助生物工艺中增强的苯酚去除。

Enhanced phenol removal in an innovative lignite activated coke-assisted biological process.

机构信息

State Environmental Protection Key Laboratory of Efficient Utilization Technology of Coal Waste Resources, Shanxi Collaborative Innovation Center of High Value-added Utilization of Coal-related Wastes, Shanxi University, Wucheng Road, Taiyuan 030006, China; Shanxi Conservancy Technical Institute, No. 2 Xinhua North Road, Taiyuan, Shanxi 030027, China.

State Environmental Protection Key Laboratory of Efficient Utilization Technology of Coal Waste Resources, Shanxi Collaborative Innovation Center of High Value-added Utilization of Coal-related Wastes, Shanxi University, Wucheng Road, Taiyuan 030006, China.

出版信息

Bioresour Technol. 2018 Jul;260:357-363. doi: 10.1016/j.biortech.2018.03.091. Epub 2018 Mar 29.

Abstract

In this study, a lignite activated coke (LAC)-assisted activated sludge (AS) process was developed for enhancing biodegradation of phenol, while the effects of LAC on sludge properties and microbial community structure were investigated. It was found that more than 90% of phenol was removed within 1 h in the LAC/AS, which was 3 times higher than the conventional AS process. Moreover, the floc size and settleability were also significantly improved in the LAC/AS. These results suggested that LAC could serve as the nucleating agent to promote the formation of compact floc, which was beneficial for toxicity mitigation and system stability. The microbial community analysis by 16S high-throughput pyrosequencing technology further revealed a more abundant bacterial richness and diversity in the LAC/AS process loaded with phenol, while some phenol degraders, such as Propionibacteriaceae were enriched. Engineering implications further suggests the LAC-assisted AS process is technically sound and economically viable.

摘要

在本研究中,开发了一种褐煤基活性炭(LAC)辅助活性污泥(AS)工艺,用于增强苯酚的生物降解,同时考察了 LAC 对污泥性质和微生物群落结构的影响。结果发现,LAC/AS 中 1 h 内去除了超过 90%的苯酚,比传统 AS 工艺高 3 倍。此外,LAC/AS 中的絮体尺寸和沉降性能也得到了显著改善。这些结果表明,LAC 可以作为成核剂促进致密絮体的形成,有利于减轻毒性和提高系统稳定性。通过 16S 高通量焦磷酸测序技术进行的微生物群落分析进一步表明,在加载苯酚的 LAC/AS 过程中,细菌丰富度和多样性更加丰富,而一些苯酚降解菌,如丙酸杆菌科被富集。工程意义进一步表明,LAC 辅助 AS 工艺在技术上是合理的,在经济上是可行的。

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