Department of Physics, University of Toronto, 60 St. George Street, Toronto, Ontario M5S 1A7, Canada.
Advanced Photon Source, Argonne National Laboratory, Argonne, Illinois 60439, USA.
Phys Rev Lett. 2018 Apr 27;120(17):177203. doi: 10.1103/PhysRevLett.120.177203.
We report a resonant inelastic x-ray scattering study of the magnetic excitation spectrum in a highly insulating Eu_{2}Ir_{2}O_{7} single crystal that exhibits a metal-insulator transition at T_{MI}=111(7) K. A propagating magnon mode with a 20 meV bandwidth and a 28 meV magnon gap is found in the excitation spectrum at 7 K, which is expected in the all-in-all-out magnetically ordered state. This magnetic excitation exhibits substantial softening as the temperature is raised towards T_{MI} and turns into a highly damped excitation in the paramagnetic phase. Remarkably, the softening occurs throughout the whole Brillouin zone including the zone boundary. This observation is inconsistent with the magnon renormalization expected in a local moment system and indicates that the strength of the electron correlation in Eu_{2}Ir_{2}O_{7} is only moderate, so that electron itinerancy should be taken into account in describing its magnetism.
我们报告了在高度绝缘的 Eu_{2}Ir_{2}O_{7}单晶中磁激发谱的共振非弹性 X 射线散射研究,该单晶在 T_{MI}=111(7) K 处表现出金属-绝缘体转变。在 7 K 的激发谱中发现了一个具有 20 meV 带宽和 28 meV 磁子能隙的传播磁子模式,这在全内全出磁有序态中是预期的。随着温度升高到 T_{MI},这种磁激发显著软化,并在顺磁相转变为高度阻尼的激发。值得注意的是,软化发生在整个布里渊区,包括区边界。这一观察结果与局域磁矩系统中预期的磁子重整化不一致,表明 Eu_{2}Ir_{2}O_{7}中的电子相关强度仅适中,因此在描述其磁性时应考虑电子巡游。