Vergara-Temprado Jesús, Holden Mark A, Orton Thomas R, O'Sullivan Daniel, Umo Nsikanabasi S, Browse Jo, Reddington Carly, Baeza-Romero María Teresa, Jones Jenny M, Lea-Langton Amanda, Williams Alan, Carslaw Ken S, Murray Benjamin J
Institute for Climate and Atmospheric Science, School of Earth and Environment University of Leeds Leeds UK.
Now at Institute for Atmospheric and Climate Science ETH Zurich Zurich Switzerland.
J Geophys Res Atmos. 2018 Apr 27;123(8):4273-4283. doi: 10.1002/2017JD027831. Epub 2018 Apr 26.
It has been hypothesized that black carbon (BC) influences mixed-phase clouds by acting as an ice-nucleating particle (INP). However, the literature data for ice nucleation by BC immersed in supercooled water are extremely varied, with some studies reporting that BC is very effective at nucleating ice, whereas others report no ice-nucleating ability. Here we present new experimental results for immersion mode ice nucleation by BC from two contrasting fuels (n-decane and eugenol). We observe no significant heterogeneous nucleation by either sample. Using a global aerosol model, we quantify the maximum relative importance of BC for ice nucleation when compared with K-feldspar and marine organic aerosol acting as INP. Based on the upper limit from our laboratory data, we show that BC contributes at least several orders of magnitude less INP than feldspar and marine organic aerosol. Representations of its atmospheric ice-nucleating ability based on older laboratory data produce unrealistic results when compared against ambient observations of INP. Since BC is a complex material, it cannot be unambiguously ruled out as an important INP species in all locations at all times. Therefore, we use our model to estimate a range of values for the density of active sites that BC particles must have to be relevant for ice nucleation in the atmosphere. The estimated values will guide future work on BC, defining the required sensitivity of future experimental studies.
据推测,黑碳(BC)作为冰核粒子(INP)会影响混合相云。然而,关于浸入过冷水的BC的冰核形成的文献数据差异极大,一些研究报告称BC在冰核形成方面非常有效,而其他研究则报告其没有冰核形成能力。在此,我们展示了来自两种截然不同的燃料(正癸烷和丁香酚)的BC在浸入模式下冰核形成的新实验结果。我们观察到两个样品均未出现显著的异质核化现象。使用全球气溶胶模型,我们量化了与作为INP的钾长石和海洋有机气溶胶相比,BC对冰核形成的最大相对重要性。基于我们实验室数据的上限,我们表明BC作为INP的贡献比长石和海洋有机气溶胶至少低几个数量级。与INP的环境观测结果相比,基于旧实验室数据对其大气冰核形成能力的表述产生了不切实际的结果。由于BC是一种复杂物质,不能在所有时间所有地点明确排除其作为重要INP物种的可能性。因此,我们使用我们的模型来估计BC颗粒对于大气中冰核形成必须具备的活性位点密度的一系列值。估计值将指导未来关于BC的研究工作,确定未来实验研究所需的灵敏度。