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神府新城不同土地利用类型多环芳烃的浓度、来源及生态风险

[Concentration, Sources and Ecological Risks of PAHs of Different Land Use Types in Shenfu New City].

作者信息

Wang Jing, Liu Ming-Li, Zhang Shi-Chao, Lu Yin-Tao, Yao Hong

机构信息

School of Civil Engineering, Beijing Jiaotong University, Beijing 100044, China.

Beijing Key Laboratory of Aqueous Typical Pollutants Control and Water Quality Safeguard, Beijing 100044, China.

出版信息

Huan Jing Ke Xue. 2017 Feb 8;38(2):703-710. doi: 10.13227/j.hjkx.201607096.

Abstract

The concentration level of polycyclic aromatic hydrocarbon (PAHs) in topsoil from Shenfu New City in urbanization was studied. 54 topsoil samples were collected from Shenfu New City and 4 different land uses (urban land, rural land, forest land, cultivated land) were included. The concentration of PAHs in different land uses was analyzed, the sources of soil PAHs were analyzed by using diagnostic ratios and principal component analysis, and the ecological risks were calculated using toxic equivalency concentrations of BaP and the incremental lifetime cancer risk(ILCR)model. Results indicated that the concentrations of ∑PAHs in urban land, cultivated land, rural land and forest land were in the range of 184-18276, 230-14102, 151-3205, 303-2980 μg·kg, respectively. Four land uses had similar sources, the main sources were coal combustion and traffic emission. According to the calculation of ecological risks, there were potential health risks for residents in Shenfu New City, especially urban land, meanwhile, residents were easily exposed to soil PAHs through dermal contact.

摘要

研究了城市化进程中神府新城表层土壤中多环芳烃(PAHs)的浓度水平。从神府新城采集了54个表层土壤样本,涵盖4种不同土地利用类型(城市用地、农村用地、林地、耕地)。分析了不同土地利用类型中PAHs的浓度,利用诊断比值和主成分分析方法分析了土壤PAHs的来源,并采用苯并[a]芘的毒性当量浓度和增量终生癌症风险(ILCR)模型计算了生态风险。结果表明,城市用地、耕地、农村用地和林地中∑PAHs的浓度分别在184 - 18276、230 - 14102、151 - 3205、303 - 2980 μg·kg范围内。四种土地利用类型的来源相似,主要来源是煤炭燃烧和交通排放。根据生态风险计算,神府新城居民存在潜在健康风险,尤其是城市用地,同时居民容易通过皮肤接触暴露于土壤PAHs中。

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