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[中国南方两个典型森林生态系统中硫、氮和汞的沉降]

[Deposition of Sulfur, Nitrogen and Mercury in Two Typical Forest Ecosystems in Southern China].

作者信息

Cheng Zheng-Lin, Luo Yao, Zhang Ting, Duan Lei

机构信息

State Key Joint Laboratory of Environmental Simulation and Pollution Control, School of Environment, Tsinghua University, Beijing 100084, China.

出版信息

Huan Jing Ke Xue. 2017 Dec 8;38(12):5004-5011. doi: 10.13227/j.hjkx.201705103.

DOI:10.13227/j.hjkx.201705103
PMID:29964558
Abstract

Bulk precipitation collectors and canopy throughfall collectors were applied to measure the deposition of sulfur, nitrogen, and mercury at two forest ecology stations, Qianyanzhou (QYZ) in Jiangxi Province and Huitong (HT) in Hunan Province, from December 2013 to November 2014. During the observation period, the volume weighted average concentrations of SO-S, NO-N, NH-N, and Hg at QYZ station were 1.89 mg·L, 0.957 mg·L, 0.401 mg·L, and 12.5 ng·L in the bulk precipitation, respectively, and 2.39 mg·L, 1.18 mg·L, 0.897 mg·L, and 22.2 ng·L in the throughfall, respectively. The concentrations of these components increased by different proportions for the bulk precipitation compared to the throughfall. At HT station, the average concentrations of SO-S, NO-N, NH-N, and Hg in the throughfall were 2.93 mg·L, 1.60 mg·L, 0.502 mg·L, and 22.0 ng·L, respectively. In addition, atmospheric deposition fluxes based on the throughfall were 3.56 g·(m·a) for sulfur, 3.02 g·(m·a) for nitrogen, and 30.6 μg·(m·a) for mercury at QYZ station, while the corresponding fluxes were 6.18 g·(m·a), 4.48 g·(m·a), and 37.3 μg·(m·a) at HT station. The deposition rates of all three elements were the highest in summer. The contribution of dry deposition to the total deposition of mercury was similar to that of wet deposition, while wet deposition contributed more to the total deposition of sulfur and nitrogen than did dry deposition. Unlike sulfur and nitrogen depositions, which were mainly derived from anthropogenic sources, mercury deposition might have a greater contribution from natural sources, especially at HT station.

摘要

2013年12月至2014年11月期间,在江西千烟洲(QYZ)和湖南会同(HT)两个森林生态站,采用大容量降水收集器和林冠穿透水收集器来测量硫、氮和汞的沉降。观测期间,QYZ站大容量降水中SO-S、NO-N、NH-N和Hg的体积加权平均浓度分别为1.89 mg·L、0.957 mg·L、0.401 mg·L和12.5 ng·L,穿透水中分别为2.39 mg·L、1.18 mg·L、0.897 mg·L和22.2 ng·L。与穿透水相比,大容量降水中这些组分的浓度以不同比例增加。在HT站,穿透水中SO-S、NO-N、NH-N和Hg的平均浓度分别为2.93 mg·L、1.60 mg·L、0.502 mg·L和22.0 ng·L。此外,基于穿透水的QYZ站硫的大气沉降通量为3.56 g·(m·a),氮为3.02 g·(m·a),汞为30.6 μg·(m·a),而HT站相应通量分别为6.18 g·(m·a)、4.48 g·(m·a)和37.3 μg·(m·a)。所有三种元素的沉降速率在夏季最高。干沉降对汞总沉降的贡献与湿沉降相似,而湿沉降对硫和氮总沉降的贡献比干沉降更大。与主要源自人为源的硫和氮沉降不同,汞沉降可能更多地来自自然源,尤其是在HT站。

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