Li Fen, Wang Xun, Luo Ji, Yuan Wei, Yu Zi-Heng, Shang Li-Hai
State Key Laboratory of Environmental Geochemistry, Institute of Geochemistry, Chinese Academy of Sciences, Guiyang 550081, China.
University of Chinese Academy of Sciences, Beijing 100049, China.
Huan Jing Ke Xue. 2017 Jul 8;38(7):3045-3053. doi: 10.13227/j.hjkx.201612089.
The rapid economy growth led to the environmental carrying capacity reaching the maximum level.Given that the time changing trend of heavy metal pollution in the remote forest ecosystems has rarely been reported, we reported the differences of Pb, Hg, Cd, As, Cr, Mn, Cu, Zn and bioaccumulation in twigs and leaves of fir() between samples collected in 1999 and 2014 at the Mt. Gongga, which was located at eastern Tibet Plateau. Our results suggested that the concentrations of Pb, Hg, As, Cd, Mn and Cu in the samples collected in 1999 were significantly higher than those collected in 2014, while the concentrations of Cr, Zn and Ba in samples collected in 2014 were higher than those collected in 1999. The correlation analysis indicated that concentrations of Pb, Hg, Cr, As, Cd, Mn, Cu, Zn and Ba in leaves were positive correlated to the age of the leaves. In addition, Hg was apt to enrich in leaves while the other metals were prone to enrich in twigs. According to the multiple linear regression result, about 70.6% of Hg in leaves and twigs was from air, while the other heavy metals, including Pb, Cr, As, Cd, Cu, Zn, and Ba, were mainly from soil(42.3%-92.2%). These results suggest that there may be different accumulation mechanisms in forest ecosystems between Hg and the other heavy metals.
经济的快速增长导致环境承载能力达到极限。鉴于偏远森林生态系统中重金属污染的时间变化趋势鲜有报道,我们报告了位于青藏高原东部贡嘎山1999年和2014年采集的样本中,冷杉嫩枝和树叶中铅、汞、镉、砷、铬、锰、铜、锌的差异及生物累积情况。我们的结果表明,1999年采集的样本中铅、汞、砷、镉、锰和铜的浓度显著高于2014年采集的样本,而2014年采集的样本中铬、锌和钡的浓度高于1999年采集的样本。相关性分析表明,树叶中铅、汞、铬、砷、镉、锰、铜、锌和钡的浓度与树叶年龄呈正相关。此外,汞易于在树叶中富集,而其他金属则倾向于在嫩枝中富集。根据多元线性回归结果,树叶和嫩枝中约70.6%的汞来自空气,而其他重金属,包括铅、铬、砷、镉、铜、锌和钡,主要来自土壤(42.3%-92.2%)。这些结果表明,森林生态系统中汞与其他重金属的累积机制可能不同。