Chen Hui, Yang Su-Ying, Li Yan-Wei, Yin Yan, Zhang Ze-Feng, Yu Xing-Na, Kang Na, Yan Shu-Qi, Xia Hang
Key Laboratory of Meteorological Disaster, Ministry of Education(KLME), Joint International Research Laboratory of Climate and Environment Change(ILCEC), Collaborative Innovation Center on Forecast and Evaluation of Meteorological Disasters(CIC-FEMD), Key Laboratory for Aerosol-Cloud-Precipitation of China Meteorological Administration, Nanjing University of Information Science and Technology, Nanjing 210044, China.
Huan Jing Ke Xue. 2016 Jun 8;37(6):2008-2016. doi: 10.13227/j.hjkx.2016.06.002.
The hygroscopic properties of aerosol have significant impact on aerosol optical properties, cloud condensation nuclei activity and human health. Aerosol particles growth factor and size-resolved ions chemical compositions were monitored in Mt. Huang. The hygroscopic properties of aerosol particles in Mt. Huang were studied. The results demonstrated that between 70 nm and 230 nm, the mass fractions of (NH)SO, organic matter and other insoluble materials were the highest. The fraction of NHNO standed in the medium. The fraction of NHHSO was the lowest. The fraction of inorganic salts increased with increasing particle diameter. Aerosol particles during daytime had stronger hygroscopicity than that at night and the hygroscopicity of aerosol became stronger when its diameter increased. The calculation hygroscopic parameter of aerosol particles showed similar diurnal variation characteristics to the observation . Good closure could be achieved when ZSR mixing rule was used based on aerosol chemical composition to calculate aerosol hygroscopic parameter and the coefficient of determination was 0.60 for all the diameters.
气溶胶的吸湿特性对气溶胶光学特性、云凝结核活性及人体健康有着重大影响。在黄山对气溶胶粒子生长因子及粒径分辨离子化学组成进行了监测,并研究了黄山气溶胶粒子的吸湿特性。结果表明,在70纳米至230纳米之间,(NH)₂SO₄、有机物及其他不溶性物质的质量分数最高,NH₄NO₃的占比处于中等水平,NH₄HSO₄的占比最低。无机盐的占比随粒径增大而增加。白天的气溶胶粒子吸湿能力强于夜间,且气溶胶粒径增大时其吸湿能力增强。气溶胶粒子的计算吸湿参数呈现出与观测相似的日变化特征。基于气溶胶化学成分采用ZSR混合规则计算气溶胶吸湿参数时可实现良好的闭合,所有粒径下的决定系数均为0.60。