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[不同湖盆入湖河流沉积物中可迁移氮形态的空间分布及影响因素]

[Spatial Distributions of Transferable Nitrogen Forms and Influencing Factors in Sediments from Inflow Rivers in Different Lake Basins].

作者信息

Zhou Rui, Yuan Xu-Yin, Marip Ja Bawk, Yu Hui-Hui, Zhang Qi, Tang Dou-Dou

机构信息

College of Environment, Hohai University, Nanjing 210098, China.

Key Laboratory of Integrated Regulation and Resource Development on Shallow Lakes, Ministry of Education, Nanjing 210098, China.

出版信息

Huan Jing Ke Xue. 2018 Mar 8;39(3):1122-1128. doi: 10.13227/j.hjkx.201706234.

Abstract

It is necessary to investigate the distribution of nitrogen forms in river sediments to recognize the water environment quality. In this study, ion exchangeable form nitrogen(IEF-N), weak acid extractable form nitrogen (WAEF-N), strong alkali extractable form nitrogen (SAEF-N) and strong oxidation extractable form nitrogen (SOEF-N) in sediments were obtained by means of sequential extraction procedures.We analyzed the spatial variations of nitrogen forms in sediments from Taihu watershed (Dongtiaoxi River and Xitiaoxi River) and Hongzehu watershed (Anhe River and Suihe River), and expounded the influence factors of nitrogen form distribution. The results showed that the physicochemical properties of sediments from different watersheds varied in space. The concentrations of total nitrogen and nitrogen fractions also showed obvious changes in river sediments. As a whole, the concentrations of total nitrogen and transferable nitrogen in Taihu rivers were higher than those in Hongzehu rivers, but the former showed smaller spatial changes. Sediments from Taihu rivers showed the different concentration order of total nitrogen and transferable nitrogen comparing with those from Hongzehu rivers. The former followed the order of SOEF-N > SAEF-N > IEF-N > WAEF-N, and the latter followed the order of SOEF-N > SAEF-N > WAEF-N > IEF-N.The spatial varitions of transferable nitrogen fractions in Hongzehu rivers were prominent, which was associated with nitrogen sources. The spatial distributions of transferable nitrogen in sediments were obviously affected by their physicochemical properties, especially for organic matter and grain size.

摘要

为了了解水环境质量,有必要研究河流沉积物中氮形态的分布。本研究采用连续提取法获得沉积物中的离子交换态氮(IEF-N)、弱酸提取态氮(WAEF-N)、强碱提取态氮(SAEF-N)和强氧化提取态氮(SOEF-N)。分析了太湖流域(东苕溪和西苕溪)和洪泽湖流域(安河和睢河)沉积物中氮形态的空间变化,并阐述了氮形态分布的影响因素。结果表明,不同流域沉积物的理化性质存在空间差异。河流沉积物中总氮和氮组分的浓度也呈现出明显变化。总体而言,太湖流域河流中总氮和可转化氮的浓度高于洪泽湖流域河流,但前者的空间变化较小。太湖流域河流沉积物与洪泽湖流域河流沉积物相比,总氮和可转化氮的浓度顺序不同。前者遵循SOEF-N>SAEF-N>IEF-N>WAEF-N的顺序,后者遵循SOEF-N>SAEF-N>WAEF-N>IEF-N的顺序。洪泽湖流域河流中可转化氮组分的空间变化较为突出,这与氮源有关。沉积物中可转化氮的空间分布明显受其理化性质的影响,尤其是有机质和粒度。

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