Pradhan Suman Kalyan, Dalal Biswajit, De S K
J Phys Condens Matter. 2018 Sep 12;30(36):365801. doi: 10.1088/1361-648X/aad7d6. Epub 2018 Aug 3.
We report the temperature and magnetic field dependent magnetic properties of the single-phase polycrystalline LaSrCrRuO sample to explore the intrinsic magnetic phases of the sample. Our combined temperature and field dependent magnetization studies reveal the formation of ferromagnetic (FM) cluster-glass in the antiferromagnetic (AFM) matrix of host LaCrO. Interestingly, the as-studied sample exhibits both zero-field-cooled (horizontal shift) and field-cooled (vertical shift) exchange bias effects and, in both cases, magnitude of exchange bias field continuously increases with the decrease of temperature. Our successive hysteresis loop measurements completely ruled out the effect of any minor hysteresis loop and thus, establishes this vertical shift as conventional field-cooled exchange bias (CEB) effect, originating from the uncompensated spins of randomly substituted canted AFM spin structure. A significantly larger value of CEB field (7.5 kOe) at 5 K is achieved for a cooling field of 50 kOe, not usually observed in conventional FM/AFM interfacial exchange-bias systems.
我们报告了单相多晶LaSrCrRuO样品的温度和磁场依赖磁性,以探索该样品的本征磁相。我们结合温度和磁场依赖的磁化研究揭示了在主体LaCrO的反铁磁(AFM)基质中形成了铁磁(FM)团簇玻璃。有趣的是,所研究的样品表现出零场冷却(水平偏移)和场冷却(垂直偏移)交换偏置效应,并且在这两种情况下,交换偏置场的大小都随着温度的降低而持续增加。我们连续的磁滞回线测量完全排除了任何微小磁滞回线的影响,因此,将这种垂直偏移确定为传统的场冷却交换偏置(CEB)效应,其源于随机取代的倾斜AFM自旋结构的未补偿自旋。对于50 kOe的冷却场,在5 K时实现了7.5 kOe的显著更大的CEB场值,这在传统的FM/AFM界面交换偏置系统中通常未观察到。