Interfaculty Institute of Biochemistry, University of Tübingen, D-72076, Tübingen, Germany.
Department of Biochemistry, University of Zurich, CH-8057, Zurich, Switzerland.
Sci Rep. 2018 Aug 28;8(1):12953. doi: 10.1038/s41598-018-31098-x.
The peptidoglycan of Staphylococcus aureus is highly amidated. Amidation of α-D-isoglutamic acid in position 2 of the stem peptide plays a decisive role in the polymerization of cell wall building blocks. S. aureus mutants with a reduced degree of amidation are less viable and show increased susceptibility to methicillin, indicating that targeting the amidation reaction could be a useful strategy to combat this pathogen. The enzyme complex that catalyzes the formation of α-D-isoglutamine in the Lipid II stem peptide was identified recently and shown to consist of two subunits, the glutamine amidotransferase-like protein GatD and the Mur ligase homolog MurT. We have solved the crystal structure of the GatD/MurT complex at high resolution, revealing an open, boomerang-shaped conformation in which GatD is docked onto one end of MurT. Putative active site residues cluster at the interface between GatD and MurT and are contributed by both proteins, thus explaining the requirement for the assembled complex to carry out the reaction. Site-directed mutagenesis experiments confirm the validity of the observed interactions. Small-angle X-ray scattering data show that the complex has a similar conformation in solution, although some movement at domain interfaces can occur, allowing the two proteins to approach each other during catalysis. Several other Gram-positive pathogens, including Streptococcus pneumoniae, Clostridium perfringens and Mycobacterium tuberculosis have homologous enzyme complexes. Combined with established biochemical assays, the structure of the GatD/MurT complex provides a solid basis for inhibitor screening in S. aureus and other pathogens.
金黄色葡萄球菌的肽聚糖高度酰胺化。位于肽聚糖骨干中第 2 位的α-D-异谷氨酸的酰胺化在细胞壁构建块的聚合中起着决定性的作用。酰胺化程度降低的金黄色葡萄球菌突变体的生存能力较低,对甲氧西林的敏感性增加,这表明靶向酰胺化反应可能是对抗这种病原体的一种有用策略。最近,催化脂质 II 骨干中α-D-异谷氨酰胺形成的酶复合物被鉴定出来,由两个亚基组成,即谷氨酰胺酰胺转移酶样蛋白 GatD 和 Mur 连接酶同源物 MurT。我们已经以高分辨率解决了 GatD/MurT 复合物的晶体结构,揭示了一种开放的、棒状构象,其中 GatD 停靠在 MurT 的一端。假定的活性位点残基聚集在 GatD 和 MurT 之间的界面处,并且由两个蛋白质贡献,从而解释了组装的复合物进行反应的要求。定点突变实验证实了观察到的相互作用的有效性。小角度 X 射线散射数据表明,该复合物在溶液中具有相似的构象,尽管在域界面处可能会发生一些运动,但在催化过程中允许两个蛋白质相互接近。其他几种革兰氏阳性病原体,包括肺炎链球菌、产气荚膜梭菌和结核分枝杆菌,都有同源的酶复合物。结合已建立的生化测定方法,GatD/MurT 复合物的结构为金黄色葡萄球菌和其他病原体的抑制剂筛选提供了坚实的基础。