Rajeev Rajendran, Hellwagner Johannes, Schumacher Anne, Jordan Inga, Huppert Martin, Tehlar Andres, Niraghatam Bhargava Ram, Baykusheva Denitsa, Lin Nan, von Conta Aaron, Wörner Hans Jakob
Laboratory of Physical Chemistry, Department of Chemistry and Applied Biosciences, Vladimir-Prelog-Weg 2, ETH Zurich, Zurich 8093, Switzerland.
Light Sci Appl. 2016 Nov 18;5(11):e16170. doi: 10.1038/lsa.2016.170. eCollection 2016 Nov.
Monochromatization of high-harmonic sources has opened fascinating perspectives regarding time-resolved photoemission from all phases of matter. Such studies have invariably involved the use of spectral filters or spectrally dispersive optical components that are inherently lossy and technically complex. Here we present a new technique for the spectral selection of near-threshold harmonics and their spatial separation from the driving beams without any optical elements. We discover the existence of a narrow phase-matching gate resulting from the combination of the non-collinear generation geometry in an extended medium, atomic resonances and absorption. Our technique offers a filter contrast of up to 10 for the selected harmonics against the adjacent ones and offers multiple temporally synchronized beamlets in a single unified scheme. We demonstrate the selective generation of 133, 80 or 56 nm femtosecond pulses from a 400-nm driver, which is specific to the target gas. These results open new pathways towards phase-sensitive multi-pulse spectroscopy in the vacuum- and extreme-ultraviolet, and frequency-selective output coupling from enhancement cavities.
高谐波源的单色化开启了关于物质所有相的时间分辨光发射的迷人前景。此类研究总是涉及使用本质上有损耗且技术复杂的光谱滤波器或光谱色散光学元件。在此,我们提出一种新技术,用于近阈值谐波的光谱选择及其与驱动光束的空间分离,且无需任何光学元件。我们发现,在扩展介质中,由于非共线产生几何结构、原子共振和吸收的组合,存在一个狭窄的相位匹配窗口。我们的技术针对所选谐波与相邻谐波提供高达10的滤波对比度,并在单一统一方案中提供多个时间同步的子光束。我们展示了从400纳米驱动源选择性产生133、80或56纳米的飞秒脉冲,这对目标气体具有特异性。这些结果为真空和极紫外波段的相敏多脉冲光谱学以及增强腔的频率选择性输出耦合开辟了新途径。