Scientific Research Academy of Guangxi Environmental Protection, Nanning 530022, China; Institute for Environmental and Climate Research, Jinan University, Guangzhou 510632, China.
Scientific Research Academy of Guangxi Environmental Protection, Nanning 530022, China.
J Environ Sci (China). 2018 Oct;72:64-74. doi: 10.1016/j.jes.2017.12.012. Epub 2017 Dec 20.
A single particle aerosol mass spectrometer was deployed to measure the changes of single particle species and sizes during March 2015 in Weizhou Island of the Beibu Gulf, Guangxi province, South China. In this campaign, a total of 3,100,597 particles were sized, and 25.8% particles with both positive and negative mass spectrum were collected and 24.8% characterized in combination with the ART-2a neural network algorithm. The distribution of sized particles was mainly in from 520 to 600nm, and the diameters ranging from 340 to 1000nm accounted for above 90%. Eight types of particles were classified: Elemental Carbon containing (EC), Organic Carbon containing (OC), EC and OC combined containing particles, Na containing particles, K containing particles (K), Levoglucosan containing particles, mineral containing particles, and Heavy Metal containing particles (HM). EC, OC and K were the major containing particles, which accounted for 84.3% in the eight types particles. The relative ratio and size distribution of the three types were EC (48.1%, 620nm), OC (12.7%, 440nm), and K (23.5%, 600nm), respectively. The three types of particles were a bit increasing ratios compared with those in clean periods during haze pollution periods. Combined with the back-trajectory results from the Hysplit-4 model and local pollution sources revealed that the ambient air quality on the Weizhou Island may be influenced by biomass burning in the Indochina Peninsula (biomass burning in the Indochina Peninsula) from the transportation on higher level atmospheric layer and by mainland of south China located northeast of Weizhou Island on the ground.
单颗粒气溶胶质谱仪被部署用于测量 2015 年 3 月在中国华南北部湾涠洲岛期间单颗粒种类和粒径的变化。在本次观测中,共测量了 3100597 个粒子,收集到正、负质量谱的粒子共有 25.8%,并结合 ART-2a 神经网络算法对其中的 24.8%的粒子进行了特征分析。所测量的粒子主要分布在 520-600nm 之间,粒径在 340-1000nm 之间的粒子占比超过 90%。共将粒子分为 8 种类型:含元素碳(EC)的粒子、含有机碳(OC)的粒子、同时含 EC 和 OC 的粒子、含钠(Na)的粒子、含钾(K)的粒子、含左旋葡聚糖(Levoglucosan)的粒子、含矿物质的粒子和含重金属(HM)的粒子。EC、OC 和 K 是主要的含粒子类型,在 8 种粒子中占比分别为 84.3%。这三种粒子的相对比例和粒径分布分别为 EC(48.1%,620nm)、OC(12.7%,440nm)和 K(23.5%,600nm)。与清洁时期相比,这三种粒子在霾污染时期的比例略有增加。结合 HYSPLIT-4 轨迹模型的后向轨迹结果和当地污染源分析表明,涠洲岛的大气环境质量可能受到来自中南半岛生物质燃烧(生物质燃烧来自中南半岛)的影响,这些污染物通过高层大气输送,以及来自中国大陆东南部、位于涠洲岛东北方向的大陆源的影响。