Physics and Physical Oceanography, Memorial University of Newfoundland, St. John's, Newfoundland, A1B 3X7 Canada.
Phys Rev E. 2018 Aug;98(2-1):022602. doi: 10.1103/PhysRevE.98.022602.
We characterize the superdiffusive dynamics of tracer particles in an electrohydrodynamically driven emulsion of oil droplets in an immiscible oil medium, where the amplitude and frequency of an external electric field are the control parameters. In the weakly driven electrohydrodynamic regime, the droplets are trapped dielectrophoretically on a patterned electrode, and the driving is therefore spatially varying. We find excellent agreement with a 〈x^{2}〉∼t^{1.5} power law and find that this superdiffusive dynamics arises from an underlying displacement distribution that is distinctly non-Gaussian and exponential for small displacements and short times. While these results are comparable with a random-velocity field model, the tracer particle speeds are in fact spatially varying in two dimensions, arising from a spatially varying electrohydrodynamic driving force. This suggests that the important ingredient for the superdiffusive t^{1.5} behavior observed is a velocity field that is isotropic in the plane and spatially correlated. Finally, we can extract, from the superdiffusive dynamics, a experimental length scale that corresponds to the lateral range of the hydrodynamic flows. This experimental length scale is non zero only above a threshold ion mobility length.
我们描述了在不相容油介质中的油滴乳液中,在外加电场的幅度和频率作为控制参数的情况下,示踪粒子的超扩散动力学。在外加电场的弱驱动电动力学状态下,液滴被介电泳捕获在图案化电极上,因此驱动是空间变化的。我们发现与〈x^{2}〉∼t^{1.5}幂律有极好的一致性,并发现这种超扩散动力学源于一个基本的位移分布,对于小位移和短时间,该分布明显是非高斯和指数的。虽然这些结果与随机速度场模型相当,但示踪粒子的速度实际上在二维空间中是变化的,这是由于空间变化的电动力学驱动力所致。这表明,观察到的超扩散 t^{1.5}行为的重要因素是各向同性的平面速度场和空间相关。最后,我们可以从超扩散动力学中提取出一个实验长度尺度,该尺度对应于流体动力学流的横向范围。只有在离子迁移率长度的阈值以上,这个实验长度尺度才不为零。