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NMR 揭示 CaK(Fe_{1-x}Ni_{x})_{4}As_{4}中刺猬自旋涡旋反铁磁量子临界点

Hedgehog Spin-Vortex Crystal Antiferromagnetic Quantum Criticality in CaK(Fe_{1-x}Ni_{x})_{4}As_{4} Revealed by NMR.

机构信息

Ames Laboratory, U.S. DOE, Ames, Iowa 50011, USA.

Department of Physics and Astronomy, Iowa State University, Ames, Iowa 50011, USA.

出版信息

Phys Rev Lett. 2018 Sep 28;121(13):137204. doi: 10.1103/PhysRevLett.121.137204.

Abstract

Two ordering states, antiferromagnetism and nematicity, have been observed in most iron-based superconductors (SCs). In contrast to those SCs, the newly discovered SC CaK(Fe_{1-x}Ni_{x}){4}As{4} exhibits an antiferromagnetic (AFM) state, called hedgehog spin-vortex crystal (SVC) structure, without nematic order, providing the opportunity for the investigation into the relationship between spin fluctuations and SC without any effects of nematic fluctuations. Our ^{75}As nuclear magnetic resonance studies on CaK(Fe_{1-x}Ni_{x}){4}As{4} (0≤x≤0.049) revealed that CaKFe_{4}As_{4} is located close to a hidden hedgehog SVC AFM quantum-critical point (QCP). The magnetic QCP without nematicity in CaK(Fe_{1-x}Ni_{x}){4}As{4} highlights the close connection of spin fluctuations and superconductivity in iron-based SCs. The advantage of stoichiometric composition also makes CaKFe_{4}As_{4} an ideal platform for further detailed investigation of the relationship between magnetic QCP and superconductivity in iron-based SCs without disorder effects.

摘要

两种有序态,反铁磁性和向列相,已在大多数铁基超导体(SCs)中观察到。与那些SCs 不同,新发现的 SC CaK(Fe_{1-x}Ni_{x}){4}As{4} 表现出反铁磁(AFM)态,称为刺猬自旋涡旋晶体(SVC)结构,没有向列序,为研究没有向列涨落影响的自旋涨落和 SC 之间的关系提供了机会。我们对 CaK(Fe_{1-x}Ni_{x}){4}As{4}(0≤x≤0.049)的 ^{75}As 核磁共振研究表明,CaKFe_{4}As_{4} 接近隐藏的刺猬 SVC AFM 量子临界点(QCP)。CaK(Fe_{1-x}Ni_{x}){4}As{4} 中没有向列性的磁性 QCP 突出了铁基SCs 中自旋涨落和超导性之间的紧密联系。化学计量组成的优势也使得 CaKFe_{4}As_{4} 成为进一步详细研究铁基 SCs 中磁性 QCP 和超导性之间关系的理想平台,而不受无序效应的影响。

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